Towards low-carbon low-energy concrete alternatives: Life cycle assessment of carbonated cementitious material-based precast panels

IF 8 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Science of the Total Environment Pub Date : 2025-04-07 DOI:10.1016/j.scitotenv.2025.179279
Dipti Kamath , Xingang Zhao , Kristina O. Armstrong , Paula Bran Anleu , Hongbin Sun , Rocio Uria Martinez , M. Parans Paranthaman
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Abstract

Cement is responsible for 22 % of all global CO2 emissions from industrial processes. Technological innovation for developing and deploying of alternative materials will be required to decarbonize the cement industry. Carbonated cementitious materials (CCMs) are building materials that rely on carbon mineralization for their strength. A process-based cradle-to-gate life cycle assessment (LCA) was conducted to evaluate the global warming potential (GWP), cumulative energy demand, and water consumption of a lab-scale CCM-based precast panel compared to a conventional precast concrete panel. Since the CCM process is currently a lab-scale early-stage process, the CCM panel showed higher environmental impacts compared to the conventional panel. However, scenario analyses include mature production process scenarios. A sensitivity analysis revealed that the GWP of CCM can be lowered to below that of the conventional panel using polymers, fillers, low-carbon electricity sources, and optimized carbonation parameters.

Extended abstract

Concrete is the second-most consumed product by weight worldwide and a significant contributor to global CO2 emissions. Cement, the critical component of concrete, is responsible for 22 % of all global CO2 emissions from industrial processes. Technological innovation for developing and deploying of alternative materials will be required to decarbonize the cement industry. Carbonated cementitious materials (CCMs) are building materials that rely on carbon mineralization for their strength. As with the development of any new technology, evaluating the environmental impacts of CCM throughout its development process is imperative to identify hotspots and ensure no unintended consequences. A process-based cradle-to-gate life cycle assessment (LCA) was conducted to evaluate the global warming potential (GWP), cumulative energy demand, and water consumption of a lab-scale CCM-based precast panel compared to a conventional precast concrete panel. Since the CCM process is currently a lab-scale early-stage process, the CCM panel showed higher environmental impacts compared to the conventional panel. The CCM panel is currently produced by curing in a lab-scale carbonation chamber for weeks, which results in high electricity consumption. However, as the production process matures, changes to the LCA results will be expected and have been incorporated into this study by scenario analysis. Multiple scenarios were considered, including reduction of electricity consumption during carbonation, change in polymer type, addition of filler materials like sand, use of renewable electricity sources, and integration of lime calcination with carbon capture and reuse for carbonation. This last scenario offers promising potential to promote circular economy practices and move towards greater sustainability. A sensitivity analysis revealed that the GWP of CCM can be lowered to below that of the conventional panel using polymers, fillers, low-carbon electricity sources, and optimized carbonation parameters.

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迈向低碳低能耗混凝土替代品:碳化胶凝材料预制板的生命周期评估
水泥占全球工业过程二氧化碳排放总量的22%。开发和部署替代材料的技术创新将需要使水泥工业脱碳。碳化胶凝材料(CCMs)是一种依靠碳矿化来增强强度的建筑材料。进行了一项基于过程的生命周期评估(LCA),以评估实验室规模的ccm预制板与传统预制混凝土板相比的全球变暖潜势(GWP)、累积能源需求和用水量。由于CCM工艺目前是实验室规模的早期工艺,与传统面板相比,CCM面板显示出更高的环境影响。然而,场景分析包括成熟的生产过程场景。灵敏度分析表明,采用聚合物、填料、低碳电源和优化的碳化参数可以将CCM的GWP降低到低于传统面板的GWP。混凝土是世界上消耗量第二大的产品,也是全球二氧化碳排放的重要贡献者。水泥是混凝土的关键成分,其排放量占全球工业过程中二氧化碳排放量的22%。开发和部署替代材料的技术创新将需要使水泥工业脱碳。碳化胶凝材料(CCMs)是一种依靠碳矿化来增强强度的建筑材料。与任何新技术的发展一样,在CCM的整个开发过程中评估其对环境的影响是必要的,以确定热点并确保没有意外后果。进行了一项基于过程的生命周期评估(LCA),以评估实验室规模的ccm预制板与传统预制混凝土板相比的全球变暖潜势(GWP)、累积能源需求和用水量。由于CCM工艺目前是实验室规模的早期工艺,与传统面板相比,CCM面板显示出更高的环境影响。CCM面板目前是通过在实验室规模的碳化室中固化数周来生产的,这导致了高电力消耗。然而,随着生产过程的成熟,LCA结果的变化将是预期的,并已通过情景分析纳入本研究。考虑了多种方案,包括减少碳化过程中的电力消耗,改变聚合物类型,添加填充材料(如沙子),使用可再生电力来源,以及将石灰煅烧与碳捕获和碳化再利用相结合。最后一种情况为促进循环经济实践和实现更大的可持续性提供了巨大的潜力。灵敏度分析表明,采用聚合物、填料、低碳电源和优化的碳化参数可以将CCM的GWP降低到低于传统面板的GWP。
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来源期刊
Science of the Total Environment
Science of the Total Environment 环境科学-环境科学
CiteScore
17.60
自引率
10.20%
发文量
8726
审稿时长
2.4 months
期刊介绍: The Science of the Total Environment is an international journal dedicated to scientific research on the environment and its interaction with humanity. It covers a wide range of disciplines and seeks to publish innovative, hypothesis-driven, and impactful research that explores the entire environment, including the atmosphere, lithosphere, hydrosphere, biosphere, and anthroposphere. The journal's updated Aims & Scope emphasizes the importance of interdisciplinary environmental research with broad impact. Priority is given to studies that advance fundamental understanding and explore the interconnectedness of multiple environmental spheres. Field studies are preferred, while laboratory experiments must demonstrate significant methodological advancements or mechanistic insights with direct relevance to the environment.
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