Flashback in diluted hydrogen flames

IF 8.3 2区 工程技术 Q1 CHEMISTRY, PHYSICAL International Journal of Hydrogen Energy Pub Date : 2025-04-09 DOI:10.1016/j.ijhydene.2025.04.029
Seunghyun Jo
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Abstract

Flashback has been studied experimentally in premixed hydrogen/air with a dilution gas. The experiments, finding a critical velocity that occurs boundary laser flashback, were conducted in a quartz glass tube with an inner diameter of 3, 4, 5, and 6 mm at the equivalence ratio between 0.6 and 3.1. N2, Ar, He, and CO2 were used as a dilution gas. The concentration of the dilution gas in the fuel mixture was 15 and 30 %. An infrared camera monitored flame development in the tube. The critical velocity gradient at the boundary of the gas stream, where the flashback is observed, has been systematically investigated and determined through experimental methods for each specific set of experimental conditions. The critical velocity gradient is independent of the tube diameter and dependent on the equivalence ratio, the dilution fraction, and the dilution gas. Generally, the magnitude of the flashback velocity gradient follows an order: undiluted hydrogen, Ar dilution, He dilution, N2 dilution, and CO2 dilution flames. The flashback velocity gradient reduces with increasing the dilution gas concentration. An experimental equation for the flashback velocity gradient indicates that the flashback at the boundary in the hydrogen flames is influenced by both the laminar flame speed and the Lewis number.
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在稀释的氢火焰中闪回
在带稀释气体的氢气/空气预混合条件下对闪回现象进行了实验研究。在内径分别为3、4、5、6 mm的石英玻璃管中,以0.6 ~ 3.1的等效比进行了边界激光闪回的临界速度实验。用N2、Ar、He和CO2作为稀释气体。混合燃料中稀释气体的浓度分别为15%和30%。红外摄像机监控着管内火焰的发展。在每一组特定的实验条件下,通过实验方法系统地研究和确定了观察到闪回的气流边界的临界速度梯度。临界流速梯度与管径无关,而与当量比、稀释分数和稀释气体有关。一般来说,闪回速度梯度的大小顺序为:未稀释的氢气、Ar稀释、He稀释、N2稀释和CO2稀释火焰。随着稀释气体浓度的增加,闪回速度梯度减小。闪回速度梯度的实验方程表明,氢火焰边界处的闪回受层流火焰速度和路易斯数的影响。
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来源期刊
International Journal of Hydrogen Energy
International Journal of Hydrogen Energy 工程技术-环境科学
CiteScore
13.50
自引率
25.00%
发文量
3502
审稿时长
60 days
期刊介绍: The objective of the International Journal of Hydrogen Energy is to facilitate the exchange of new ideas, technological advancements, and research findings in the field of Hydrogen Energy among scientists and engineers worldwide. This journal showcases original research, both analytical and experimental, covering various aspects of Hydrogen Energy. These include production, storage, transmission, utilization, enabling technologies, environmental impact, economic considerations, and global perspectives on hydrogen and its carriers such as NH3, CH4, alcohols, etc. The utilization aspect encompasses various methods such as thermochemical (combustion), photochemical, electrochemical (fuel cells), and nuclear conversion of hydrogen, hydrogen isotopes, and hydrogen carriers into thermal, mechanical, and electrical energies. The applications of these energies can be found in transportation (including aerospace), industrial, commercial, and residential sectors.
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