Gas Sensor Drift Compensation Using Semi-Supervised Ensemble Classifiers with Multi-Level Features and Center Loss.

IF 9.1 1区 化学 Q1 CHEMISTRY, ANALYTICAL ACS Sensors Pub Date : 2025-04-25 Epub Date: 2025-04-08 DOI:10.1021/acssensors.4c03655
Kai Jiang, Min Zeng, Tao Wang, Yu Wu, Wangze Ni, Lechen Chen, Jianhua Yang, Nantao Hu, Bowei Zhang, Fuzhen Xuan, Siying Li, Anwei Shi, Zhi Yang
{"title":"Gas Sensor Drift Compensation Using Semi-Supervised Ensemble Classifiers with Multi-Level Features and Center Loss.","authors":"Kai Jiang, Min Zeng, Tao Wang, Yu Wu, Wangze Ni, Lechen Chen, Jianhua Yang, Nantao Hu, Bowei Zhang, Fuzhen Xuan, Siying Li, Anwei Shi, Zhi Yang","doi":"10.1021/acssensors.4c03655","DOIUrl":null,"url":null,"abstract":"<p><p>The drift compensation of gas sensors is a significant and challenging issue in the field of electronic noses (E-nose). Compensating sensor drift has a great benefit in improving the performance of E-nose systems. However, conventional methods often perform poorly due to complex data relationships before and after drifting, or require label information for both nondrift (source data) and drift data (target data) to enhance performance, which is hard to achieve and even unrealistic. In this study, we propose a semisupervised domain adaptive convolutional neural network (CNN) based on ensemble classifiers of multilevel features, pretraining, and center loss to tackle the drift problem. The main idea is to make full use of multilevel features extracted from the network and apply Hilbert space's maximum mean discrepancy (MMD) to evaluate the domain similarity of the features at different levels. Then the corresponding MMD is used as a weight to achieve the weighted fusion of predictions in the classifier ensemble module, so as to obtain a more reliable result. Furthermore, to optimize training, MMD is used as a loss for pretraining to help feature extractors learn more robust and common features in two domains. Center loss is also applied to achieve more focused learning for features of the same class. The results on two data sets demonstrate the effectiveness of our method. The average classification accuracies under different settings reach 76.06% (long-drift) and 82.07% (short-drift), respectively, and the average <i>R</i><sup>2</sup> score reaches 0.804 in the regression task, which has significant improvements compared with several conventional methods. Our work provides an effective and reliable method at the algorithm level to solve the drift compensation problem of gas sensors.</p>","PeriodicalId":24,"journal":{"name":"ACS Sensors","volume":" ","pages":"2906-2918"},"PeriodicalIF":9.1000,"publicationDate":"2025-04-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Sensors","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1021/acssensors.4c03655","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/4/8 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
引用次数: 0

Abstract

The drift compensation of gas sensors is a significant and challenging issue in the field of electronic noses (E-nose). Compensating sensor drift has a great benefit in improving the performance of E-nose systems. However, conventional methods often perform poorly due to complex data relationships before and after drifting, or require label information for both nondrift (source data) and drift data (target data) to enhance performance, which is hard to achieve and even unrealistic. In this study, we propose a semisupervised domain adaptive convolutional neural network (CNN) based on ensemble classifiers of multilevel features, pretraining, and center loss to tackle the drift problem. The main idea is to make full use of multilevel features extracted from the network and apply Hilbert space's maximum mean discrepancy (MMD) to evaluate the domain similarity of the features at different levels. Then the corresponding MMD is used as a weight to achieve the weighted fusion of predictions in the classifier ensemble module, so as to obtain a more reliable result. Furthermore, to optimize training, MMD is used as a loss for pretraining to help feature extractors learn more robust and common features in two domains. Center loss is also applied to achieve more focused learning for features of the same class. The results on two data sets demonstrate the effectiveness of our method. The average classification accuracies under different settings reach 76.06% (long-drift) and 82.07% (short-drift), respectively, and the average R2 score reaches 0.804 in the regression task, which has significant improvements compared with several conventional methods. Our work provides an effective and reliable method at the algorithm level to solve the drift compensation problem of gas sensors.

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
基于多级特征和中心损失的半监督集成分类器的气体传感器漂移补偿。
气体传感器的漂移补偿是电子鼻领域的一个重要而富有挑战性的问题。补偿传感器漂移对提高电子鼻系统的性能有很大的好处。然而,由于漂移前后的数据关系复杂,传统的方法往往性能不佳,或者需要非漂移数据(源数据)和漂移数据(目标数据)的标签信息来提高性能,这很难实现,甚至不现实。在这项研究中,我们提出了一种基于多层特征集成分类器、预训练和中心损失的半监督域自适应卷积神经网络(CNN)来解决漂移问题。其主要思想是充分利用从网络中提取的多层特征,利用希尔伯特空间的最大平均差异(MMD)来评价不同层次特征的域相似度。然后将相应的MMD作为权重,在分类器集成模块中实现预测的加权融合,从而获得更可靠的结果。此外,为了优化训练,将MMD用作预训练的损失,以帮助特征提取器在两个域中学习更鲁棒和通用的特征。中心损失也被用于对同一类的特征进行更集中的学习。在两个数据集上的结果证明了该方法的有效性。不同设置下的平均分类准确率分别达到76.06%(长漂移)和82.07%(短漂移),回归任务的平均R2得分达到0.804,与几种常规方法相比有显著提高。本文的工作在算法层面上为解决气体传感器漂移补偿问题提供了一种有效、可靠的方法。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
ACS Sensors
ACS Sensors Chemical Engineering-Bioengineering
CiteScore
14.50
自引率
3.40%
发文量
372
期刊介绍: ACS Sensors is a peer-reviewed research journal that focuses on the dissemination of new and original knowledge in the field of sensor science, particularly those that selectively sense chemical or biological species or processes. The journal covers a broad range of topics, including but not limited to biosensors, chemical sensors, gas sensors, intracellular sensors, single molecule sensors, cell chips, and microfluidic devices. It aims to publish articles that address conceptual advances in sensing technology applicable to various types of analytes or application papers that report on the use of existing sensing concepts in new ways or for new analytes.
期刊最新文献
Visible Light-Rectified Chemiresistive Sensing in Two-Dimensional Conductive Metal-Organic Frameworks Multifunctional Wearable OLED−OPD System with Wavelength-Tunable Emission for Phototheranostics High-Performance SERS Detection of Monoamine Neurotransmitters Using a Nanogap-Engineered Plasmonic Platform with Application to Human Plasma Metal-Organic Framework-Based and Humidity-Tolerant Quartz Crystal Microbalance Sensor for Difluoromethane Refrigerant Leak Detection. Humidity-Independent NO2 Gas Sensors Based on CeO2/ZnO/WO3 Heterostructure Films Fabricated by Template-Assisted Magnetron Sputtering
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1