Investigation on the Chaotic Mixing Mechanism of High-Viscosity Fluids with Laminar Flow in an Irregular Impeller Stirred Tank

IF 3.9 3区 工程技术 Q2 ENGINEERING, CHEMICAL Industrial & Engineering Chemistry Research Pub Date : 2025-04-08 DOI:10.1021/acs.iecr.5c00008
Deyin Gu, Changshu Li, Yinghua Song, Hui Xu, Ting yao
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Abstract

In this work, an impeller with a fractal structure design was introduced in the laminar mixing of high-viscosity fluids to facilitate chaotic advection. Power consumption characteristics, mixing time, Kolmogorov entropy, and 0–1 test were applied to characterize the mixing performance and chaotic mixing characteristics. Visualization experiment, Poincaré section, and trajectories of massless particles were employed to investigate the structure of the flow field. The findings showed that the fractal structure design introduced in the impeller blades provided a reduction in power consumption, power number, and mixing time and an improvement in the Kolmogorov entropy and chaotic mixing degree, while additional energy conservation, less mixing time, and a higher chaotic mixing degree were achieved by increasing the fractal iteration number in the impeller blades. Poincaré section showed the isolated mixing regions (IMRs) and chaotic mixing regions (CMRs) in the flow field, and the phenomenon can also be confirmed by visualization experiment. The particles within the IMRs did not undergo material exchange but rather exhibited movement solely within the designated regions. In addition, the trajectories of massless particles suggested that the fractal structure design of impeller blades facilitated structural instability of the IMRs, stimulated fluid particles to escape from the IMRs into the CMRs, and induced chaotic advection in the flow field.

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非规则叶轮搅拌槽内高粘度流体层流混沌混合机理研究
本文在高粘度流体层流混合中引入了分形结构的叶轮,以促进混沌平流。采用功耗特性、混合时间、Kolmogorov熵和0-1检验对混合性能和混沌混合特性进行表征。采用可视化实验、庞加莱剖面和无质量粒子轨迹对流场结构进行了研究。研究结果表明,叶轮叶片分形结构设计降低了功率消耗、功率数和混合时间,提高了Kolmogorov熵和混沌混合程度,增加叶轮叶片分形迭代次数可以实现额外的能量节约,减少了混合时间,提高了混沌混合程度。poincar截面显示了流场中的孤立混合区(IMRs)和混沌混合区(CMRs),这一现象也可以通过可视化实验得到证实。imr内的粒子不进行物质交换,而只在指定区域内运动。此外,无质量颗粒的运动轨迹表明,叶轮叶片的分形结构设计加剧了内腔结构的不稳定性,刺激流体颗粒从内腔逃逸到cmr中,并在流场中引起混沌平流。
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来源期刊
Industrial & Engineering Chemistry Research
Industrial & Engineering Chemistry Research 工程技术-工程:化工
CiteScore
7.40
自引率
7.10%
发文量
1467
审稿时长
2.8 months
期刊介绍: ndustrial & Engineering Chemistry, with variations in title and format, has been published since 1909 by the American Chemical Society. Industrial & Engineering Chemistry Research is a weekly publication that reports industrial and academic research in the broad fields of applied chemistry and chemical engineering with special focus on fundamentals, processes, and products.
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