Modeling of ceramic hollow fiber membrane self-heated with electrical current for oxygen separation from air

IF 9 1区 工程技术 Q1 ENGINEERING, CHEMICAL Journal of Membrane Science Pub Date : 2025-04-08 DOI:10.1016/j.memsci.2025.124088
Hamed Abdolahimansoorkhani, Xingjian Xue
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Abstract

Oxygen permeation process through a gas-tight mixed conducting membrane is thermally activated in nature. To maintain elevated temperatures for membrane operations, a high temperature furnace is usually utilized. This leads to low efficiencies for heating power utilization and is difficult to change the temperature fast way due to the high volume of the furnace. Recently, a novel strategy has been employed to directly apply external electrical power to a hollow fiber membrane, achieving self-heating in a compact way. To better understand the fundamental mechanisms, herein, a mathematical model is developed for self-heated hollow fiber oxygen separation membrane assisted with vacuum conditions applied at the outlet of lumen side. Comprehensive simulations are conducted to study self-heating effects on Multiphysics transport processes and oxygen permeation performance. Simulations are also performed to investigate the effects of the orientations of electrical fields applied to hollow fiber membrane and the vacuum levels applied to the outlet of lumen side. The associated fundamental mechanisms are discussed and elaborated.

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电流自热陶瓷中空纤维膜与空气中氧分离的建模
氧通过气密混合导电膜的渗透过程本质上是热激活的。为了保持膜操作的高温,通常使用高温炉。这导致加热功率利用效率低,并且由于炉的体积大,难以快速改变温度。最近,一种新颖的策略被采用,直接向中空纤维膜施加外部电源,以紧凑的方式实现自加热。为了更好地理解其基本机理,本文建立了自热中空纤维氧分离膜在腔侧出口施加真空条件下的数学模型。综合模拟研究了自热对多物理场输运过程和氧渗透性能的影响。模拟研究了施加在中空纤维膜上的电场方向和施加在管腔侧出口的真空度的影响。讨论并阐述了相关的基本机制。
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来源期刊
Journal of Membrane Science
Journal of Membrane Science 工程技术-高分子科学
CiteScore
17.10
自引率
17.90%
发文量
1031
审稿时长
2.5 months
期刊介绍: The Journal of Membrane Science is a publication that focuses on membrane systems and is aimed at academic and industrial chemists, chemical engineers, materials scientists, and membranologists. It publishes original research and reviews on various aspects of membrane transport, membrane formation/structure, fouling, module/process design, and processes/applications. The journal primarily focuses on the structure, function, and performance of non-biological membranes but also includes papers that relate to biological membranes. The Journal of Membrane Science publishes Full Text Papers, State-of-the-Art Reviews, Letters to the Editor, and Perspectives.
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