Infrared Metaplasmonics

IF 6.7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Photonics Pub Date : 2025-04-15 DOI:10.1021/acsphotonics.5c00147
Zarko Sakotic, Noah Mansfeld, Amogh Raju, Alexander Ware, Divya Hungund, Daniel Krueger, Daniel Wasserman
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Abstract

Plasmonic response in metals, defined as the ability to support subwavelength confinement of surface plasmon modes, is typically limited to a narrow frequency range below the metals’ plasma frequency. This places severe limitations on the operational wavelengths of plasmonic materials and devices. However, when the volume of a metal film is massively decreased, highly confined quasi-two-dimensional surface plasmon modes can be supported out to wavelengths well beyond the plasma wavelength. While this has, thus far, been achieved using ultrathin (nm-scale) metals, such films are quite difficult to realize and suffer from even higher losses than bulk plasmonic films. To extend the plasmonic response to the infrared, here we introduce the concept of metaplasmonics, representing a novel plasmonic modality with a host of appealing properties. By fabricating and characterizing a series of metaplasmonic nanoribbons, we demonstrate large confinement, high-quality factors, and large near-field enhancements across a broad wavelength range, extending well beyond the limited bandwidth of traditional plasmonic materials. We demonstrate 35× plasmon wavelength reduction, and numerical simulations suggest that further wavelength reduction, up to a factor of 150, is achievable using our approach. The demonstration of the metaplasmonics paradigm offers a promising path to fill the near- and mid-infrared technological gap for high-quality plasmonic materials and provides a new material system to study the effects of extreme plasmonic confinement for applications in nonlinear and quantum plasmonics.

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红外Metaplasmonics
金属中的等离子体响应,定义为支持表面等离子体模式亚波长限制的能力,通常限制在金属等离子体频率以下的狭窄频率范围内。这对等离子体材料和器件的工作波长造成了严重的限制。然而,当金属薄膜的体积大量减小时,高度受限的准二维表面等离子体模式可以被支持到远超过等离子体波长的波长。虽然到目前为止,这是使用超薄(纳米级)金属实现的,但这种薄膜很难实现,并且比体等离子体薄膜遭受更高的损耗。为了将等离子体响应扩展到红外,我们在这里引入了元等离子体的概念,它代表了一种具有许多吸引人的特性的新型等离子体模态。通过制造和表征一系列的超等离子体纳米带,我们展示了在宽波长范围内的大约束、高质量因子和大的近场增强,远远超出了传统等离子体材料的有限带宽。我们证明了35倍的等离子体波长减少,数值模拟表明,进一步的波长减少,高达150的因素,是可以实现的,使用我们的方法。元等离子体范式的证明为填补高质量等离子体材料的近红外和中红外技术空白提供了一条有希望的途径,并为研究极端等离子体约束效应在非线性和量子等离子体中的应用提供了新的材料体系。
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来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
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