Fundamental mechanisms of discontinuous deformation in metals for cryogenic-environment applications

IF 9.3 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Acta Materialia Pub Date : 2025-06-15 Epub Date: 2025-04-02 DOI:10.1016/j.actamat.2025.120970
You Sub Kim , Taeuk Kang , Soon-Ku Hong , Jamieson Brechtl , Mikhail Lebyodkin , Yi-Hsuan Cheng , E-Wen Huang , Peter K. Liaw , Stefanus Harjo , Wu Gong , Ching-Yu Chiang , Soo Yeol Lee
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Abstract

Metallic materials are known to exhibit low-temperature discontinuous deformation (i.e., low-temperature serrated deformation, LTSD) at cryogenic temperatures, which can lead to sudden failures or catastrophic accidents. Therefore, understanding LTSD is crucial for ensuring material stability and reliability in a cryogenic environment. Thus far, the widely accepted explanations for the origins of LTSD can be categorized into two mechanisms: (i) dislocation-based mechanical instability and (ii) thermomechanical instability. However, interpreting LTSD using each theory independently has limitations in clearly elucidating the LTSD mechanism. Therefore, the current understanding of LTSD remains insufficient and is still subject to debate because it is challenging to prove experimentally. To address this issue, we suggest a novel LTSD mechanism, namely a thermally induced dislocation dynamics model, based on the experimental evidence that considers both the dislocation dynamics and thermomechanical characteristics at cryogenic temperatures. Furthermore, we present a modified deformation-mechanism map of a SS316L that incorporates the newly proposed LTSD mechanisms. The origin of LTSD is considered in the unique framework of dislocation behavior under severely limited thermal-vibration energy at cryogenic temperatures, leading to the dislocation avalanches and development of hierarchical dislocation networks, including multiple lattice defects. Therewith, the localized heating generated from dislocation avalanches induces multiple types of LTSD and gives rise to transitions from the heterogeneous to homogeneous deformation. Our findings highlight the rate-dependent nature of LTSD and negative strain-rate sensitivity in the strength-elongation relationship and include the first observation of changes in small stress fluctuations and their relationship to the changes in larger serrations.

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低温环境下金属不连续变形的基本机制
已知金属材料在低温下表现出低温不连续变形(即低温锯齿形变形,LTSD),这可能导致突然失效或灾难性事故。因此,了解LTSD对于确保材料在低温环境中的稳定性和可靠性至关重要。迄今为止,对LTSD起源的广泛接受的解释可以分为两种机制:(i)基于位错的机械不稳定性和(ii)热机械不稳定性。然而,单独使用每种理论解释LTSD在清楚阐明LTSD机制方面存在局限性。因此,目前对LTSD的理解仍然不足,并且由于实验证明具有挑战性,因此仍然存在争议。为了解决这一问题,我们提出了一种新的LTSD机制,即基于实验证据的热诱导位错动力学模型,该模型同时考虑了低温下的位错动力学和热力学特性。此外,我们提出了一个改进的SS316L的变形机制图,其中包含了新提出的LTSD机制。LTSD的起源被认为是在低温下严重有限的热振动能量下的位错行为的独特框架下,导致位错雪崩和分层位错网络的发展,包括多个晶格缺陷。因此,位错雪崩产生的局部加热诱发了多种类型的LTSD,并导致了非均质变形向均质变形的转变。我们的研究结果强调了LTSD的速率依赖性质和负应变率敏感性在强度-延伸关系中,包括首次观察到小应力波动的变化及其与大锯齿变化的关系。
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来源期刊
Acta Materialia
Acta Materialia 工程技术-材料科学:综合
CiteScore
16.10
自引率
8.50%
发文量
801
审稿时长
53 days
期刊介绍: Acta Materialia serves as a platform for publishing full-length, original papers and commissioned overviews that contribute to a profound understanding of the correlation between the processing, structure, and properties of inorganic materials. The journal seeks papers with high impact potential or those that significantly propel the field forward. The scope includes the atomic and molecular arrangements, chemical and electronic structures, and microstructure of materials, focusing on their mechanical or functional behavior across all length scales, including nanostructures.
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