Fast photophysical processes of a single NV center modulated by the near-infrared laser pulse

IF 3.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Applied Physics Letters Pub Date : 2025-04-16 DOI:10.1063/5.0254845
Yujing Cao, Yan Liu, Junjie Lin, Mengting He, Xinrui Yuan, Botao Wu, E. Wu
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Abstract

The photophysics of the nitrogen-vacancy (NV) center in diamond has been extensively investigated. Especially the fast optical switch based on the NV centers' photoluminescence (PL) by the near-infrared laser (NIR) modulation has been demonstrated, but the photophysical processes behind it are still not fully understood. Here, the NIR modulation on the PL of an isolated single NV center in bulk diamond is probed and detected with precision at picosecond timescale. We thereby observe NIR optical excitation at the NV ground state as well as at the excited state. Meanwhile, a generalized model is constructed with additional energy levels that can be reached under NIR illumination. The transition rates from numerical simulations are demonstrated in good agreement with the experimental results. Our findings may provide insights into the understanding of the NV center's related photophysics and open intriguing prospects such as reversible optical switching, super-resolution microscopy, and so forth.
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近红外激光脉冲调制单NV中心的快速光物理过程
金刚石中氮空位(NV)中心的光物理性质得到了广泛的研究。特别是基于近红外激光调制NV中心的光致发光(PL)的快速光开关已经被证实,但其背后的光物理过程仍未完全了解。本文在皮秒时间尺度上,对块体金刚石中孤立的单NV中心的PL上的近红外调制进行了探测和精确检测。因此,我们观察到近红外光激发在近红外基态和激发态。同时,建立了一个广义模型,其中包含了近红外光照下可达到的附加能级。数值模拟结果与实验结果吻合较好。我们的发现可能会为了解NV中心的相关光物理学提供见解,并开辟有趣的前景,如可逆光开关,超分辨率显微镜等。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Applied Physics Letters
Applied Physics Letters 物理-物理:应用
CiteScore
6.40
自引率
10.00%
发文量
1821
审稿时长
1.6 months
期刊介绍: Applied Physics Letters (APL) features concise, up-to-date reports on significant new findings in applied physics. Emphasizing rapid dissemination of key data and new physical insights, APL offers prompt publication of new experimental and theoretical papers reporting applications of physics phenomena to all branches of science, engineering, and modern technology. In addition to regular articles, the journal also publishes invited Fast Track, Perspectives, and in-depth Editorials which report on cutting-edge areas in applied physics. APL Perspectives are forward-looking invited letters which highlight recent developments or discoveries. Emphasis is placed on very recent developments, potentially disruptive technologies, open questions and possible solutions. They also include a mini-roadmap detailing where the community should direct efforts in order for the phenomena to be viable for application and the challenges associated with meeting that performance threshold. Perspectives are characterized by personal viewpoints and opinions of recognized experts in the field. Fast Track articles are invited original research articles that report results that are particularly novel and important or provide a significant advancement in an emerging field. Because of the urgency and scientific importance of the work, the peer review process is accelerated. If, during the review process, it becomes apparent that the paper does not meet the Fast Track criterion, it is returned to a normal track.
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