Plastic additives in the diet: Occurrence and dietary exposure in different population groups

IF 11.3 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Journal of Hazardous Materials Pub Date : 2025-08-05 Epub Date: 2025-04-17 DOI:10.1016/j.jhazmat.2025.138317
Julio Fernández-Arribas, Teresa Moreno, Ethel Eljarrat
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Abstract

A total diet study focused on exposure to plastic additives has been performed on 109 food samples. Plasticizers were detected in 85 % of analyzed samples with total concentrations ranging between not detected (nd) and 22.0 µg/g wet weight (ww). Non-phthalate plasticizers (NPPs), such as acetyl tributyl citrate (ATBC) or di(2-ethylhexyl) adipate (DEHA), were detected predominantly in baby foods (nd-3.38 µg/g ww) and meat (nd-15.0 µg/g ww), respectively. Significant differences (p ≤ 0.001) were observed across foods with different packaging types regarding the presence of ATBC and DEHA. ATBC was primarily detected in foods packaged in glass containers, meanwhile DEHA is mainly related to fresh food wrapped in plastic materials. Additionally, transference assays in selected ready to cook meals and fresh vegetables were performed, with NPPs exhibiting a higher transference from packaging to food than other compounds. The data obtained have been used for an assessment of estimated daily intake (EDI) of plastic additives in infants (6–12 months), toddlers (1–3 years), and adults (>18 years), resulting in values ranging 0.29–516 µg/kg body weight (bw)/day. Human risk related to baby food consumption, expressed as hazard quotients (HQs), was found with di(2-ethylhexyl) phthalate (DEHP) in the infant population sub-group.

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饮食中的塑料添加剂:在不同人群中的发生和饮食暴露
对109个食品样本进行了一项以塑料添加剂暴露为重点的全面饮食研究。85%的分析样品中检测到增塑剂,总浓度范围在未检测到(nd)和22.0µg/g湿重(ww)之间。非邻苯二甲酸酯增塑剂(NPPs),如乙酰柠檬酸三丁酯(ATBC)或己酸二(2-乙基己基)二(DEHA),主要在婴儿食品中检测到(nd-3.38µg/g ww)。肉(nd-15.0µg/g ww)。在不同包装类型的食品中观察到ATBC和DEHA存在显著差异(p≤0.001)。ATBC主要在玻璃包装的食品中检测到,DEHA主要在塑料包装的新鲜食品中检测到。此外,在选定的即食饭菜和新鲜蔬菜中进行了转移试验,与其他化合物相比,NPPs从包装到食物的转移率更高。所获得的数据已用于评估婴儿(6-12个月)、幼儿(1-3岁)和成人(18岁)塑料添加剂的估计每日摄入量(EDI),得出的数值范围为0.29-516µg/kg体重(bw)/天。与婴儿食品消费相关的人类风险,以危险商(hq)表示,在婴儿人群亚组中发现邻苯二甲酸二(2-乙基己基)酯(DEHP)。
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来源期刊
Journal of Hazardous Materials
Journal of Hazardous Materials 工程技术-工程:环境
CiteScore
25.40
自引率
5.90%
发文量
3059
审稿时长
58 days
期刊介绍: The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.
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