Following Charge Carrier Transport in Freestanding Core–Shell GaN Nanowires on n-Si(111) Substrates

IF 4.7 3区 材料科学 Q1 ENGINEERING, ELECTRICAL & ELECTRONIC ACS Applied Electronic Materials Pub Date : 2025-04-01 DOI:10.1021/acsaelm.5c00198
Juliane Koch, Patrick Häuser, Peter Kleinschmidt, Lisa Liborius, Nils Weimann and Thomas Hannappel*, 
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Abstract

Well-defined heterojunctions inside nanostructured device structures are a basic requirement for any nanoscale device design with advanced electrical properties. For the evaluation of the desired functionalities on the nanoscale, a study of the electrical behavior with appropriate spatial resolution is highly revealing. We specifically address GaN-based core–shell heterostructures and perform multiprobe measurements with ultrahigh spatial resolution. The n+-GaN nanowire core exhibits favorable electrical conductivity, and the behavior of charge carrier transport at a n+-nonintentionally doped -n+-doped core–shell double heterojunction is demonstrated when applying an electron beam-induced current mode. This investigation offers direct insights into the selective charge carrier transport, and therefore into the rectifying junction within the core–shell GaN nanowire, and contributes to a model of the conductivity channels. This experimental approach is crucial for any future advancement of device structures that incorporate bottom-up-grown, heterostructure core–shell GaN nanowires on conductive Si(111) substrates.

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跟踪 n-Si(111)基底上独立核壳氮化镓纳米线中的电荷载流子传输
纳米结构器件结构内部定义明确的异质结是任何具有先进电气特性的纳米级器件设计的基本要求。为了评估纳米尺度上所需的功能,研究具有适当空间分辨率的电学行为极具启发性。我们特别针对基于氮化镓的核壳异质结构,进行了具有超高空间分辨率的多探针测量。n+-GaN 纳米线内核表现出良好的导电性,在应用电子束诱导电流模式时,n+-无意掺杂-n+-掺杂核壳双异质结的电荷载流子传输行为得到了证实。这项研究直接揭示了电荷载流子的选择性传输,从而揭示了核壳氮化镓纳米线内的整流结,并有助于建立导电通道模型。这种实验方法对于未来在导电硅(111)衬底上采用自下而上生长的异质结构核壳氮化镓纳米线的器件结构的发展至关重要。
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来源期刊
CiteScore
7.20
自引率
4.30%
发文量
567
期刊介绍: ACS Applied Electronic Materials is an interdisciplinary journal publishing original research covering all aspects of electronic materials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials science, engineering, optics, physics, and chemistry into important applications of electronic materials. Sample research topics that span the journal's scope are inorganic, organic, ionic and polymeric materials with properties that include conducting, semiconducting, superconducting, insulating, dielectric, magnetic, optoelectronic, piezoelectric, ferroelectric and thermoelectric. Indexed/​Abstracted: Web of Science SCIE Scopus CAS INSPEC Portico
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