Structure and propagation of spherical turbulent iron-methane hybrid flame at elevated pressure

IF 5.8 2区 工程技术 Q2 ENERGY & FUELS Combustion and Flame Pub Date : 2023-09-01 DOI:10.1016/j.combustflame.2023.112918
Xiao Cai , Shouguo Su , Limin Su , Jinhua Wang , Marcus Alden , Zhongshan Li , Zuohua Huang
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Abstract

In this communication we demonstrate the role of turbulence intensity in the dual-front structure and self-similar propagation of spherical turbulent iron-methane hybrid flames. We first show that iron-methane hybrid mixture, whose iron concentration is below a critical threshold for the formation of a dust flame front in laminar or weak turbulent environment, can be burned strongly with both separated dual-front and merged single-front structures in intense turbulence. It is suggested that the formation of iron flame front would be attributed to local iron concentration accumulation by preferential sampling with near-unity Stocks number (St), heat transfer enhancement of iron particles to fluid and mixing promotion of iron particles with oxidants by strong turbulence. The propagation of iron front falls behind the methane front in the leading segments which is promoted by flame stretch for sub-unity Lewis number (Le), thus the separated dual-front structure occurs. Furthermore, the strong self-similar propagation of spherical turbulent iron-methane hybrid flame was observed under different turbulence intensities (urms). Mechanistically, such strong self-similar propagation of the hybrid flame is the consequence of the couple effects of flame mode transition at high urms with near-unity St and differential diffusion for sub-unity Le.

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球形湍流铁-甲烷混合火焰在高压下的结构与传播
在本文中,我们证明了湍流强度在球形湍流铁-甲烷混合火焰的双锋面结构和自相似传播中的作用。我们首先发现,在层流或弱湍流环境中,铁浓度低于形成粉尘火焰锋的临界阈值的铁-甲烷混合气,在强湍流环境中,无论是分离的双锋面结构还是合并的单锋面结构,都能强烈燃烧。分析认为,铁火焰锋的形成可能是由于近统一库屯数(St)的优先取样使局部铁浓度积累、强湍流增强铁颗粒对流体的传热和促进铁颗粒与氧化剂的混合。在亚单位路易斯数(Le)下,由于火焰拉伸的推动,铁锋在前段的传播落后于甲烷锋,从而形成分离的双锋结构。此外,在不同湍流强度(urms)下,观察到球形湍流铁-甲烷混合火焰的强自相似传播。从机理上讲,混合火焰的这种强自相似传播是近单位温度下火焰模态跃迁和亚单位温度下火焰微分扩散耦合作用的结果。
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来源期刊
Combustion and Flame
Combustion and Flame 工程技术-工程:化工
CiteScore
9.50
自引率
20.50%
发文量
631
审稿时长
3.8 months
期刊介绍: The mission of the journal is to publish high quality work from experimental, theoretical, and computational investigations on the fundamentals of combustion phenomena and closely allied matters. While submissions in all pertinent areas are welcomed, past and recent focus of the journal has been on: Development and validation of reaction kinetics, reduction of reaction mechanisms and modeling of combustion systems, including: Conventional, alternative and surrogate fuels; Pollutants; Particulate and aerosol formation and abatement; Heterogeneous processes. Experimental, theoretical, and computational studies of laminar and turbulent combustion phenomena, including: Premixed and non-premixed flames; Ignition and extinction phenomena; Flame propagation; Flame structure; Instabilities and swirl; Flame spread; Multi-phase reactants. Advances in diagnostic and computational methods in combustion, including: Measurement and simulation of scalar and vector properties; Novel techniques; State-of-the art applications. Fundamental investigations of combustion technologies and systems, including: Internal combustion engines; Gas turbines; Small- and large-scale stationary combustion and power generation; Catalytic combustion; Combustion synthesis; Combustion under extreme conditions; New concepts.
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