A comprehensive review on synthesis and applications of single crystal perovskite halides

IF 9.1 2区化学 Q1 CHEMISTRY, INORGANIC & NUCLEAR Progress in Solid State Chemistry Pub Date : 2020-12-01 DOI:10.1016/j.progsolidstchem.2020.100286

Sandeep Arya , Prerna Mahajan , Ramashanker Gupta , Ritu Srivastava , Naveen kumar Tailor , Soumitra Satapathi , R. Radhakrishnan Sumathi , Ram Datt , Vinay Gupta

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引用次数: 58

Abstract

Halide based perovskite materials have fascinated strong attention for being a hopeful candidate for optoelectronic device applications. Single-crystalline halide perovskites exhibit no grain boundaries and possess low trap densities; and are therefore likely to show superior optoelectronic performances in comparison to their polycrystalline film counterparts. In spite of this, their basic perceptive of physico-chemical properties are however controversial to the scientific society. In this review article, we present the deep insight into all the reported protocols available for the synthesis of purely inorganic as well as hybrid halide perovskites (incorporating organic as well as inorganic cation) to achieve high-quality single crystals. On account of advanced characteristics like long carrier recombination lifetime and exciton diffusion length, wide-ranging visible to NIR absorption, high charge mobility, controllable optoelectronic properties etc., hybrid halide perovskites have emerged to be a tough challenger in the optoelectronic research area in comparison to the purely inorganic halide perovskites and have consequently been paid much attention. Therefore, the optoelectronic properties and convenient applications of particularly hybrid halide single-crystal perovskites in various optoelectronic devices like solar cell, laser, high energy ray detector, photodetector, light-emitting diode, etc are highlighted.

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钙钛矿卤化物单晶的合成及应用综述

卤化物基钙钛矿材料作为光电子器件应用的有希望的候选者而引起了人们的强烈关注。单晶卤化物钙钛矿无晶界，陷阱密度低;因此，与它们的多晶薄膜相比，它们可能表现出优越的光电性能。尽管如此，他们对物理化学性质的基本认识在科学界还是有争议的。在这篇综述文章中，我们深入介绍了所有可用于合成纯无机和杂化卤化物钙钛矿(结合有机和无机阳离子)的报道方案，以获得高质量的单晶。杂化卤化物钙钛矿具有载流子复合寿命长、激子扩散长度长、可见光到近红外吸收范围广、电荷迁移率高、光电性能可控等先进特性，与纯无机卤化物钙钛矿相比，已成为光电研究领域一个强有力的挑战者，受到了广泛的关注。因此，特别是杂化卤化物单晶钙钛矿在太阳能电池、激光器、高能射线探测器、光电探测器、发光二极管等各种光电器件中的光电性能和便捷应用得到了突出的体现。

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来源期刊

Progress in Solid State Chemistry 化学-无机化学与核化学

CiteScore

14.10

自引率

3.30%

发文量

期刊介绍： Progress in Solid State Chemistry offers critical reviews and specialized articles written by leading experts in the field, providing a comprehensive view of solid-state chemistry. It addresses the challenge of dispersed literature by offering up-to-date assessments of research progress and recent developments. Emphasis is placed on the relationship between physical properties and structural chemistry, particularly imperfections like vacancies and dislocations. The reviews published in Progress in Solid State Chemistry emphasize critical evaluation of the field, along with indications of current problems and future directions. Papers are not intended to be bibliographic in nature but rather to inform a broad range of readers in an inherently multidisciplinary field by providing expert treatises oriented both towards specialists in different areas of the solid state and towards nonspecialists. The authorship is international, and the subject matter will be of interest to chemists, materials scientists, physicists, metallurgists, crystallographers, ceramists, and engineers interested in the solid state.