Development of picosecond time-resolved X-ray absorption spectroscopy by high-repetition-rate laser pump/X-ray probe at Beijing Synchrotron Radiation Facility

IF 3 3区 物理与天体物理 Journal of Synchrotron Radiation Pub Date : 2017-03-24 DOI:10.1107/S1600577517003277
Hao Wang, Can Yu, Xu Wei, Zhenhua Gao, Guang-Lei Xu, Da-Rui Sun, Zhenjie Li, Yangfan Zhou, Qiu-Ju Li, Bing-Bing Zhang, Jin-Qiang Xu, Lin Wang, Yan Zhang, Ying-Lei Tan, Ye Tao
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引用次数: 12

Abstract

A new setup and commissioning of transient X-ray absorption spectroscopy are described, based on the high-repetition-rate laser pump/X-ray probe method, at the 1W2B wiggler beamline at the Beijing Synchrotron Radiation Facility. A high-repetition-rate and high-power laser is incorporated into the setup with in-house-built avalanche photodiodes as detectors. A simple acquisition scheme was applied to obtain laser-on and laser-off signals simultaneously. The capability of picosecond transient X-ray absorption spectroscopy measurement was demonstrated for a photo-induced spin-crossover iron complex in 6 mM solution with 155 kHz repetition rate.

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北京同步辐射设施高重复率激光泵浦/ x射线探针的皮秒时间分辨x射线吸收光谱研究
介绍了一种基于高重复率激光泵浦/ x射线探针方法的瞬态x射线吸收光谱在北京同步辐射设施1W2B摆动光束线上的新设置和调试。一个高重复率和高功率激光器被整合到装置中,内部建造的雪崩光电二极管作为探测器。采用一种简单的采集方案同时获取激光开、关信号。用皮秒瞬态x射线吸收光谱测量了6 mM溶液中光诱导自旋交叉铁配合物,重复频率为155 kHz。
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来源期刊
Journal of Synchrotron Radiation
Journal of Synchrotron Radiation INSTRUMENTS & INSTRUMENTATIONOPTICS&-OPTICS
CiteScore
5.60
自引率
12.00%
发文量
289
审稿时长
1 months
期刊介绍: Synchrotron radiation research is rapidly expanding with many new sources of radiation being created globally. Synchrotron radiation plays a leading role in pure science and in emerging technologies. The Journal of Synchrotron Radiation provides comprehensive coverage of the entire field of synchrotron radiation and free-electron laser research including instrumentation, theory, computing and scientific applications in areas such as biology, nanoscience and materials science. Rapid publication ensures an up-to-date information resource for scientists and engineers in the field.
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