Utilization of fruit waste for H2-rich syngas production via steam co-gasification with brown coal

IF 6.4 3区 环境科学与生态学 Q2 ENERGY & FUELS Carbon Resources Conversion Pub Date : 2023-04-12 DOI:10.1016/j.crcon.2023.04.002
Aisikaer Anniwaer , Nichaboon Chaihad , Aghietyas Choirun Az Zahra , Irwan Kurnia , Yutaka Kasai , Suwadee Kongparakul , Chanatip Samart , Katsuki Kusakabe , Abuliti Abudula , Guoqing Guan
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引用次数: 1

Abstract

In this work, to efficiently utilize waste fruit and low-rank coal for the hydrogen (H2)-rich syngas production, steam co-gasification of banana peel (BP) and brown coal (BC) was studied in a fixed-bed reactor. The results showed that the gasification rate of BC was highly enhanced after mixing it with BP and the obvious synergistic effect was observed in all investigated three mixing weight ratios (i.e., 1:1, 1:4, 4:1), resulting in a higher carbon conversion as well as a H2-rich gas production yield for the co-gasification. However, the extent of promotion by synergistic effect was affected by the reaction temperature, mixing ratio, and steam amount. It was found that the high potassium (K) species content in the BP provided the catalytic effect not only on water–gas shift reaction but also on tar reforming/cracking, thereby enhancing the gasification of BC. In addition, it is confirmed that steam should be an important factor to promote the synergistic effect and H2-rich gas production.

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利用水果废弃物与褐煤蒸汽共气化生产富H2合成气
为了高效利用废水果和低阶煤生产富氢合成气,在固定床反应器上对香蕉皮(BP)和褐煤(BC)的蒸汽共气化进行了研究。结果表明,BC与BP混合后气化率显著提高,且3种混合质量比(1:1、1:4、4:1)均表现出明显的协同效应,使得共气化的碳转化率和富h2产气量均有所提高。而协同效应的促进程度受反应温度、混合比和蒸汽量的影响。结果表明,BP中钾(K)的高含量不仅对水煤气转换反应有催化作用,而且对焦油重整/裂化也有催化作用,从而促进了BC的气化。此外,还证实了蒸汽是促进协同效应和富h2产气的重要因素。
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来源期刊
Carbon Resources Conversion
Carbon Resources Conversion Materials Science-Materials Science (miscellaneous)
CiteScore
9.90
自引率
11.70%
发文量
36
审稿时长
10 weeks
期刊介绍: Carbon Resources Conversion (CRC) publishes fundamental studies and industrial developments regarding relevant technologies aiming for the clean, efficient, value-added, and low-carbon utilization of carbon-containing resources as fuel for energy and as feedstock for materials or chemicals from, for example, fossil fuels, biomass, syngas, CO2, hydrocarbons, and organic wastes via physical, thermal, chemical, biological, and other technical methods. CRC also publishes scientific and engineering studies on resource characterization and pretreatment, carbon material innovation and production, clean technologies related to carbon resource conversion and utilization, and various process-supporting technologies, including on-line or off-line measurement and monitoring, modeling, simulations focused on safe and efficient process operation and control, and process and equipment optimization.
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Outside Front Cover Outside Back Cover Developments and challenges on enhancement of photocatalytic CO2 reduction through photocatalysis Outside Front Cover Outside Back Cover
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