Effects of two-phase periodic velocity on droplet coalescence inside microchannels

IF 2 4区 化学 Q3 CHEMISTRY, MULTIDISCIPLINARY Journal of Flow Chemistry Pub Date : 2023-02-07 DOI:10.1007/s41981-023-00258-0
Wen-qing Li, Xiao-juan Li, An-qi Guan, Zhi-jiang Jin, Jin-yuan Qian
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引用次数: 1

Abstract

A novel method based on periodic change of two-phase velocity for the droplet coalescence in microchannels is proposed. The feasibility of the method is justified by investigating the droplet coalescence in several combinations of the velocity pairs. Once the droplet pairs have been generated, the frequency of the droplet coalescence can be divided into a liquid slug of continuous phase dominated region and a real velocity ratio dominated region. Since the liquid slug between the droplet pairs and the real velocity ratio of the droplet pairs are determined by the flow rate ratios, the critical value of the flow rate ratio is determined to distinguish whether the frequency of the droplet coalescence is liquid slug dominated or real velocity ratio dominated. Compared with the traditional passive method, the droplet pairs are alternatively generated by the periodic change of the two-phase velocity. The velocity gradient of the droplet pairs can be generated spontaneously which avoids the introduction of an expansion structure. The mixing performance inside the coalesced droplet is improved due to the reorganized inner circulation when the droplets is coalesced. The quantitative mixing of the reagents can be achieved to satisfy special application needs by a precise control of the volume of the droplet pairs.

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两相周期速度对微通道内液滴聚结的影响
提出了一种基于两相速度周期变化的微通道液滴聚结新方法。通过对几种速度对组合下液滴聚结的研究,证明了该方法的可行性。一旦形成液滴对,液滴聚结的频率可分为连续相主导区和实速度比主导区。由于液滴对之间的液塞和液滴对的实际速度比是由流速比决定的,因此确定流速比的临界值来区分液滴聚结频率是以液塞塞为主还是以实际速度比为主。与传统的被动方法相比,该方法利用两相速度的周期性变化交替产生液滴对。液滴对的速度梯度可以自发产生,从而避免了膨胀结构的引入。由于液滴凝聚过程中内部循环的重新组织,提高了凝聚液滴内部的混合性能。通过精确控制液滴对的体积,可以实现试剂的定量混合,以满足特殊应用的需要。
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来源期刊
Journal of Flow Chemistry
Journal of Flow Chemistry CHEMISTRY, MULTIDISCIPLINARY-
CiteScore
6.40
自引率
3.70%
发文量
29
审稿时长
>12 weeks
期刊介绍: The main focus of the journal is flow chemistry in inorganic, organic, analytical and process chemistry in the academic research as well as in applied research and development in the pharmaceutical, agrochemical, fine-chemical, petro- chemical, fragrance industry.
期刊最新文献
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