Investigation of the interface behavior of a viscous fluid under free surface shear flow using an eccentric transparent Couette cell

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2022-11-09 DOI:10.1515/ipp-2022-4261
P. Thirunavukkarasu, F. Fournier, A. Pignolet, R. Castellani, C. Cohen, E. Peuvrel-Disdier, R. Valette, B. Vergnes
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Abstract

Abstract In the present work, a prototype was developed to observe the flow behavior of viscous fluids under free surface shear and determine an adhesion energy in this flow geometry. The geometry consists of an eccentric Couette cell (outer cylinder radius of 89.5 mm, inner cylinder radius of 43.75 mm and minimal gap of 3 mm) that can be used in two modes, where both cylinders can respectively rotate in the same or opposite directions. Cylinders are horizontal and short relatively to their diameters (30 mm long). Transparent windows allow in-situ flow observations. The design, development, and testing of the prototype with a model viscous fluid (silicone fluid with a 2.2 104 Pa.s Newtonian viscosity) are reported in this paper. The flow behavior of small fluid volumes (fill factor smaller than 15%) was investigated under co- and counter-rotating configurations to determine steady-state flow conditions. Stationary conditions were identified in the counter-rotating mode. The velocity conditions and resulting observations are studied and analysed. However, for the used silicone fluid, the bulk dissipative energy is much larger than the work of adhesive forces in the investigated regimes. The adhesion energy contribution could not be detected for this fluid.
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用偏心透明Couette单元研究粘性流体在自由表面剪切流动下的界面行为
在本工作中,开发了一个原型来观察粘性流体在自由表面剪切下的流动行为,并确定该流动几何形状下的粘附能。几何结构包括一个偏心的Couette电池(外圆柱体半径89.5 mm,内圆柱体半径43.75 mm,最小间隙为3 mm),可以在两种模式下使用,其中两个圆柱体分别可以在相同或相反的方向上旋转。汽缸是水平的,相对于它们的直径(30毫米长)来说是短的。透明窗口允许现场流动观察。设计、开发和测试了一种粘性流体模型(硅胶流体,压力为2.2 104 Pa)。本文报道了牛顿黏度(牛顿黏度)。研究了小体积流体(填充系数小于15%)在共旋转和反旋转配置下的流动特性,以确定稳态流动条件。确定了逆旋转模式下的稳态条件。对速度条件和观测结果进行了研究和分析。然而,对于所使用的有机硅流体,在所研究的制度下,体积耗散能远远大于粘接力的功。无法检测到该流体的粘附能贡献。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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