G. Jang, Hyowon Han, Sunihl Ma, Junwoo Lee, Chang Uk Lee, Woo-Yang Jeong, J. Son, Dongki Cho, Ji‐Hee Kim, Cheolmin Park, Jooho Moon
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引用次数: 4
Abstract
Abstract. Perovskite light-emitting diodes (PeLEDs) are considered as promising candidates for next-generation solution-processed full-color displays. However, the external quantum efficiencies (EQEs) and operational stabilities of deep-blue (<460 nm) PeLEDs still lag far behind their red and green counterparts. Herein, a rapid crystallization method based on hot-antisolvent bathing is proposed for realization of deep-blue PeLEDs. By promoting immediate removal of the precursor solvent from the wet perovskite films, development of the quasi-two-dimensional (2D) Ruddlesden–Popper perovskite (2D-RPP) crystals with n values >3 is hampered completely, so that phase-pure 2D-RPP films with bandgaps suitable for deep-blue PeLEDs can be obtained successfully. The uniquely developed rapid crystallization method also enables formation of randomly oriented 2D-RPP crystals, thereby improving the transfer and transport kinetics of the charge carriers. Thus, high-performance deep-blue PeLEDs emitting at 437 nm with a peak EQE of 0.63% are successfully demonstrated. The color coordinates are confirmed to be (0.165, 0.044), which match well with the Rec.2020 standard blue gamut and have excellent spectral stability.
期刊介绍:
Advanced Photonics is a highly selective, open-access, international journal that publishes innovative research in all areas of optics and photonics, including fundamental and applied research. The journal publishes top-quality original papers, letters, and review articles, reflecting significant advances and breakthroughs in theoretical and experimental research and novel applications with considerable potential.
The journal seeks high-quality, high-impact articles across the entire spectrum of optics, photonics, and related fields with specific emphasis on the following acceptance criteria:
-New concepts in terms of fundamental research with great impact and significance
-State-of-the-art technologies in terms of novel methods for important applications
-Reviews of recent major advances and discoveries and state-of-the-art benchmarking.
The journal also publishes news and commentaries highlighting scientific and technological discoveries, breakthroughs, and achievements in optics, photonics, and related fields.