Steam cracker facilities in the United States: operations, emissions, and sociodemographic patterns of surrounding populations

N. Johnson, M. Bell, Nicholas Perez, Robert Dubrow, N. Deziel
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Abstract

Background: Production of shale gas in the United States (US) increased more than 10-fold from 2008 to 2021, yielding greater quantities of hydrocarbon feedstocks and incentivizing expansion of petrochemical facilities. Steam crackers (SCs) convert hydrocarbon feedstocks into ethylene and propylene (the building blocks of plastics), while releasing toxic chemicals and greenhouse gases (GHGs). Analyses of environmental health and justice impacts of SCs are limited. Methods: We described SC operations, locations, and emissions, and evaluated sociodemographic characteristics of populations residing near SCs to better understand potential public health hazards and inform future studies. We summarized and described industry-reported emissions from the US Environmental Protection Agency’s Toxic Release Inventory and GHG Reporting Program. We compared population characteristics of US Census block groups ⩽5 km and >5 km from a steam cracker-containing facility (SCF) within the same county. Results: We identified 32 SCFs across five US states, with most in Texas and Louisiana. Toxic chemicals with the greatest reported cumulative air emissions in 1987–2019 were: ethylene, propylene, hydrochloric acid, benzene, n-hexane, 1,3-butadiene, ammonia, toluene, vinyl acetate, and methanol. Reported total annual GHG emissions were 4% higher in 2019 versus 2010, with total GHG emissions of >650 million metric tons (carbon dioxide equivalents) in 2010–2019. We found that 752 465 people live in census block groups ⩽5 km from an SCF, regardless of county. Compared to block groups >5 km away within the same county, block groups closer to SCFs had statistically significantly lower median incomes ($54 843 vs $67 866) and more vacant housing (15% vs 11%), and higher proportions of residents who were non-Hispanic Black (31% vs 19%) and unemployed (8% vs 6%). Conclusion: SCs emit substantial amounts of GHGs and toxic chemicals in locations with historically disadvantaged populations. Future research could further evaluate the accuracy of reported emissions, conduct monitoring in proximate communities, and assess population-level health impacts.
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美国的蒸汽裂解装置:操作、排放和周围人口的社会人口结构模式
背景:从2008年到2021年,美国页岩气产量增长了10多倍,产生了更多的碳氢化合物原料,并激励了石化设施的扩张。蒸汽裂解器(SC)将碳氢化合物原料转化为乙烯和丙烯(塑料的组成部分),同时释放有毒化学物质和温室气体。SC对环境健康和司法影响的分析有限。方法:我们描述了SC的操作、位置和排放,并评估了居住在SC附近的人群的社会人口学特征,以更好地了解潜在的公共卫生危害,并为未来的研究提供信息。我们总结并描述了美国环境保护局有毒物质排放清单和GHG报告计划中的行业报告排放量。我们比较了同一县内距离蒸汽裂解器容纳设施(SCF)5公里和>5公里的美国人口普查区块群的人口特征。结果:我们在美国五个州发现了32个SCF,其中大部分在德克萨斯州和路易斯安那州。1987年至2019年报告的累计空气排放量最大的有毒化学品是:乙烯、丙烯、盐酸、苯、正己烷、1,3-丁二烯、氨、甲苯、乙酸乙烯酯和甲醇。与2010年相比,2019年报告的年度温室气体排放总量增加了4%,2010-2019年温室气体总排放量超过6.5亿吨(二氧化碳当量)。我们发现752 465人居住在人口普查区块群中,距离SCF 5公里,不分县。与同一县内>5公里外的街区组相比,更接近SCF的街区组的中位收入在统计上显著较低(54美元 843对67美元 866)和更多的空置住房(15%对11%),非西班牙裔黑人(31%对19%)和失业者(8%对6%)的比例更高。结论:在历史上处于不利地位的地区,SCs排放大量的温室气体和有毒化学物质。未来的研究可以进一步评估报告的排放量的准确性,在邻近社区进行监测,并评估人口水平的健康影响。
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