Displacement Patterns of a Newtonian Fluid by a Shear‐Thinning Fluid in a Rough Fracture

IF 4.6 1区 地球科学 Q2 ENVIRONMENTAL SCIENCES Water Resources Research Pub Date : 2023-09-01 DOI:10.1029/2023WR034958
Le Zhang, Zhibing Yang, Y. Méheust, I. Neuweiler, R. Hu, Yi‐Feng Chen
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Abstract

Two‐phase flow involving non‐Newtonian fluids in fractured media is of vital importance in many natural processes and subsurface engineering applications, such as rock grouting, groundwater remediation, and enhanced oil recovery. Yet, how the displacement dynamics is impacted by the non‐Newtonian rheology remains an open question. Here, we conduct primary drainage experiments in which a shear‐thinning Xanthan gum solution displaces a silicone oil in a transparent rough fracture for a wide range of shear‐thinning property (controlled by polymer concentration) and flow rates. We first evaluate the effects of shear‐thinning property on displacement efficiency. Based on qualitative and quantitative analyses of the observed fluid morphologies, we present an experimental phase diagram of the obtained displacement patterns. We characterize a novel displacement pattern where the fluid‐fluid interface changes from stable (plug flow) to unstable (fingering) as the fracture aperture, averaged over the transverse direction, varies along the mean flow direction. We demonstrate that the existence of this mixed displacement pattern can be explained by local viscosity heterogeneity induced by the coupling of the shear‐thinning behavior and the spatial variability of apertures. Finally, we propose a theoretical model elucidating the mechanisms behind the flow regime transitions. The interface stability criterion predicted by this model exhibits good agreement with the experimental measurements, and stresses the potentially important role of fluid rheology, coupled to aperture variability, in immiscible displacements in rough fractures. These findings provide new insights into the dynamics of immiscible two‐phase flows with non‐Newtonian effects, and has potential implications for the aforementioned engineering applications.
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粗糙裂缝中剪切稀化流体对牛顿流体的驱替模式
裂隙介质中非牛顿流体的两相流在许多自然过程和地下工程应用中至关重要,如岩石灌浆、地下水修复和提高石油采收率。然而,位移动力学如何受到非牛顿流变学的影响仍然是一个悬而未决的问题。在这里,我们进行了初步排水实验,其中剪切稀化黄原胶溶液置换透明粗糙裂缝中的硅油,以获得广泛的剪切稀化性能(由聚合物浓度控制)和流速。我们首先评估了剪切减薄特性对驱油效率的影响。在对观察到的流体形态进行定性和定量分析的基础上,我们给出了所获得的位移模式的实验相图。我们描述了一种新的位移模式,其中随着横向平均裂缝孔径沿平均流动方向变化,流体-流体界面从稳定(塞流)变为不稳定(指进)。我们证明,这种混合驱替模式的存在可以用剪切减薄行为和孔隙空间变异性的耦合引起的局部粘度不均匀性来解释。最后,我们提出了一个理论模型来解释流态转变背后的机制。该模型预测的界面稳定性标准与实验测量结果吻合良好,并强调了流体流变学与孔隙变异性在粗糙裂缝中不混溶位移中的潜在重要作用。这些发现为具有非牛顿效应的不混溶两相流的动力学提供了新的见解,并对上述工程应用具有潜在意义。
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来源期刊
Water Resources Research
Water Resources Research 环境科学-湖沼学
CiteScore
8.80
自引率
13.00%
发文量
599
审稿时长
3.5 months
期刊介绍: Water Resources Research (WRR) is an interdisciplinary journal that focuses on hydrology and water resources. It publishes original research in the natural and social sciences of water. It emphasizes the role of water in the Earth system, including physical, chemical, biological, and ecological processes in water resources research and management, including social, policy, and public health implications. It encompasses observational, experimental, theoretical, analytical, numerical, and data-driven approaches that advance the science of water and its management. Submissions are evaluated for their novelty, accuracy, significance, and broader implications of the findings.
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