Micro-Batch flow reactor for the photoproduction of H2O2 from water/real seawater

IF 2 4区 化学 Q3 CHEMISTRY, MULTIDISCIPLINARY Journal of Flow Chemistry Pub Date : 2023-04-19 DOI:10.1007/s41981-023-00257-1
Aswin Gopakumar, Tong Zhang, Shoubhik Das
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引用次数: 1

Abstract

Photocatalytic generation of H2O2 with heterogeneous catalysts has attracted much attentions and impressive strategies have been used to increase the photocatalytic efficiency. However, applications of these strategies to large scale are still underdeveloped. For this reason, development of flow photocatalytic strategy is highly necessary. Considering this, we have developed a serial micro-batch flow reactor for the generation of H2O2 which could easily scale up the reaction to1L scale with high reproducibility with the modified g-C3N4. With this flow reactor, the generated concentration of H2O2 has been reached to 6.89 mM and 5.89 mM in pure water and seawater, respectively.

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光处理水/真海水中H2O2的微批流反应器
非均相催化剂光催化生成H2O2的研究受到了广泛的关注,人们采用了许多有效的方法来提高光催化效率。然而,这些策略的大规模应用仍不发达。因此,开发流动光催化策略是非常有必要的。考虑到这一点,我们开发了一种用于生成H2O2的串联微批流动反应器,该反应器可以很容易地将反应规模扩大到1l规模,并且使用改性的g-C3N4具有很高的重现性。采用该流动反应器,在纯水和海水中H2O2的生成浓度分别达到6.89 mM和5.89 mM。图形抽象
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来源期刊
Journal of Flow Chemistry
Journal of Flow Chemistry CHEMISTRY, MULTIDISCIPLINARY-
CiteScore
6.40
自引率
3.70%
发文量
29
审稿时长
>12 weeks
期刊介绍: The main focus of the journal is flow chemistry in inorganic, organic, analytical and process chemistry in the academic research as well as in applied research and development in the pharmaceutical, agrochemical, fine-chemical, petro- chemical, fragrance industry.
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