Effects of Cooling System Boundary Conditions on the Performance of Proton Exchange Membrane Fuel Cell: A Comprehensive Analysis

IF 2.7 4区 工程技术 Q3 ELECTROCHEMISTRY Journal of Electrochemical Energy Conversion and Storage Pub Date : 2023-07-25 DOI:10.1115/1.4063016
Yaochen Wang, H. Ren, Cong Li
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Abstract

We developed a three-dimensional multiphysics numerical model of a Proton Exchange Mem-brane Fuel Cell (PEMFC) with a cathode mesh structure to investigate how coolant flow rate and temperature impact its performance. After experimentally validating the model, we compared the performance of the cathode mesh structure PEMFC with that of the traditional straight flow PEMFC. The results indicate that the cathode mesh structure PEMFC has a lower pressure drop and a more index of uniform distribution (IUD), leading to enhanced performance, better temperature distribution, and improved water management of the PEMFC. The investigation of the cooling system's operating parameters revealed that the temperature of the cathode catalyst layer in the PEMFC is the highest, while the temperature of the bipolar plate is the lowest. Of the nine cases that we evaluated, Case 7, with a coolant inlet temperature and flow rate of 303.15 K and 0.07 m s−1, respectively, yielded the highest power density and the lowest average temperature. The IUD of the PEM in Case 5 was 0.608, suggesting that the temperature distribution of the PEM is more uniform when the coolant inlet temperature and flow rate are 323.15 K and 0.05 m s−1, respectively. We have demonstrated through calculations that there is a strong correlation between temperature difference and IUDs. These findings have significant implications for the optimization and application of PEMFCs.
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冷却系统边界条件对质子交换膜燃料电池性能影响的综合分析
我们开发了一个具有阴极网格结构的质子交换膜燃料电池(PEMFC)的三维多物理数值模型,以研究冷却剂流速和温度如何影响其性能。在对模型进行实验验证后,我们将阴极网状结构的PEMFC与传统的直流PEMFC的性能进行了比较。结果表明,阴极网状结构的PEMFC具有更低的压降和更多的均匀分布指数(IUD),从而提高了PEMFC的性能、更好的温度分布和改进的水管理。对冷却系统运行参数的研究表明,PEMFC中阴极催化剂层的温度最高,而双极板的温度最低。在我们评估的九种情况中,冷却液入口温度和流速分别为303.15 K和0.07 m s−1的情况7产生了最高的功率密度和最低的平均温度。案例5中PEM的IUD为0.608,表明当冷却剂入口温度和流速分别为323.15 K和0.05 m s−1时,PEM的温度分布更加均匀。我们已经通过计算证明,温差和宫内节育器之间有很强的相关性。这些发现对PEMFC的优化和应用具有重要意义。
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来源期刊
CiteScore
4.90
自引率
4.00%
发文量
69
期刊介绍: The Journal of Electrochemical Energy Conversion and Storage focuses on processes, components, devices and systems that store and convert electrical and chemical energy. This journal publishes peer-reviewed archival scholarly articles, research papers, technical briefs, review articles, perspective articles, and special volumes. Specific areas of interest include electrochemical engineering, electrocatalysis, novel materials, analysis and design of components, devices, and systems, balance of plant, novel numerical and analytical simulations, advanced materials characterization, innovative material synthesis and manufacturing methods, thermal management, reliability, durability, and damage tolerance.
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