Lithium-ion battery degradation trajectory early prediction with synthetic dataset and deep learning

IF 14.9 1区 化学 Q1 Energy Journal of Energy Chemistry Pub Date : 2023-10-01 DOI:10.1016/j.jechem.2023.06.036
Mingqiang Lin , Yuqiang You , Jinhao Meng , Wei Wang , Ji Wu , Daniel-Ioan Stroe
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引用次数: 2

Abstract

Knowing the long-term degradation trajectory of Lithium-ion (Li-ion) battery in its early usage stage is critical for the maintenance of the battery energy storage system (BESS) in reality. Previous battery health diagnosis methods focus on capacity and state of health (SOH) estimation which can receive only the short-term health status of the cell. This paper proposes a novel degradation trajectory prediction method with synthetic dataset and deep learning, which enables to grasp the characterization of the cell’s health at a very early stage of Li-ion battery usage. A transferred convolutional neural network (CNN) is chosen to finalize the early prediction target, and the polynomial function based synthetic dataset generation strategy is designed to reduce the costly data collection procedure in real application. In this thread, the proposed method needs one full lifespan data to predict the overall degradation trajectories of other cells. With only the full lifespan cycling data from 4 cells and 100 cycling data from each cell in experimental validation, the proposed method shows a good prediction accuracy on a dataset with more than 100 commercial Li-ion batteries.

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基于合成数据集和深度学习的锂离子电池退化轨迹早期预测
了解锂离子电池在早期使用阶段的长期退化轨迹对于实际中电池储能系统的维护至关重要。以前的电池健康诊断方法侧重于容量和健康状态(SOH)估计,其只能接收电池的短期健康状态。本文提出了一种新的基于合成数据集和深度学习的退化轨迹预测方法,该方法能够在锂离子电池使用的早期阶段掌握电池健康状况的特征。选择转移卷积神经网络(CNN)来确定早期预测目标,并设计了基于多项式函数的合成数据集生成策略,以减少实际应用中昂贵的数据收集过程。在这个线程中,所提出的方法需要一个完整的寿命数据来预测其他细胞的整体退化轨迹。在实验验证中,只有来自4个电池的全寿命循环数据和来自每个电池的100个循环数据,该方法在具有100多个商用锂离子电池的数据集上显示出良好的预测精度。
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来源期刊
Journal of Energy Chemistry
Journal of Energy Chemistry CHEMISTRY, APPLIED-CHEMISTRY, PHYSICAL
CiteScore
19.10
自引率
8.40%
发文量
3631
审稿时长
15 days
期刊介绍: The Journal of Energy Chemistry, the official publication of Science Press and the Dalian Institute of Chemical Physics, Chinese Academy of Sciences, serves as a platform for reporting creative research and innovative applications in energy chemistry. It mainly reports on creative researches and innovative applications of chemical conversions of fossil energy, carbon dioxide, electrochemical energy and hydrogen energy, as well as the conversions of biomass and solar energy related with chemical issues to promote academic exchanges in the field of energy chemistry and to accelerate the exploration, research and development of energy science and technologies. This journal focuses on original research papers covering various topics within energy chemistry worldwide, including: Optimized utilization of fossil energy Hydrogen energy Conversion and storage of electrochemical energy Capture, storage, and chemical conversion of carbon dioxide Materials and nanotechnologies for energy conversion and storage Chemistry in biomass conversion Chemistry in the utilization of solar energy
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