Formation mechanism of NO2 distribution heterogeneity at different spatial scales

IF 12.4 Q1 ENVIRONMENTAL SCIENCES Resources Environment and Sustainability Pub Date : 2023-06-01 DOI:10.1016/j.resenv.2022.100106
Hancong Zhu , Li Yang
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引用次数: 1

Abstract

NO2 is one of the main pollutants in the atmospheric environment, which can directly or indirectly cause harm to human health. Jiangsu province is economically developed and densely populated, and the conflict between economic development and ecological environment protection is more prominent, which causes its mean annual NO2 concentration to be higher than other neighboring provinces. The study takes the formation mechanism of NO2 concentration distribution heterogeneity at different spatial scales as the research object. By using OMI satellite remote sensing data and NO2 concentration ground monitoring data in Jiangsu Province from 2015 to 2020, the paper studies NO2 concentration distribution heterogeneity at macroscopic and microscopic scales, respectively, to analyze the formation mechanism. The results show that: (1) The spatial distribution characteristics of NO2 concentration obtained based on the analysis of two data sources have good consistency, with the overall performance of high NO2 concentration in the south of Jiangsu where the concentration of NO2 column reached 16.3 × 1015 molec/cm 2 and the monitoring concentration reached 46.3μg/m3, while the concentration of NO2 in central Jiangsu is relatively low, with average concentrations of 6 × 1015 molec/cm 2 and 26μg/m3. (2) Under the macroscopic spatial scale, the average NO2 column concentration in the south of Jiangsu is 9 × 1015 molec/cm 2 higher and the monitoring concentration is 15μg/m3 than that in the north of Jiangsu; natural factors such as temperature are the important influencing factors for the heterogeneity of NO2 concentration distribution under this scale. (3) At the microscopic spatial scale, NO2 concentration is 5–10% higher in industrial concentrations in southern Jiangsu, some heating cities in northern Jiangsu, and industrial parks in northern Jiangsu. In addition, NO2 concentration decreases gradually with distance from this area; anthropogenic factors such as population density, GDP, and car ownership are important factors to influence the heterogeneity of NO2 concentration distribution at this scale. Based on the above findings, the paper proposes to adjust the industrial structure, limit the number of high energy-consuming and high-emission enterprises, and develop seasonal emission reduction measures.

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不同空间尺度NO2分布异质性的形成机制
NO2是大气环境中的主要污染物之一,可直接或间接对人体健康造成危害。江苏省经济发达,人口密集,经济发展与生态环境保护的矛盾较为突出,导致其年均NO2浓度高于周边省份。本研究以不同空间尺度下NO2浓度分布异质性的形成机制为研究对象。利用2015 - 2020年江苏省OMI卫星遥感数据和NO2浓度地面监测数据,分别在宏观和微观尺度上研究NO2浓度分布不均一性,分析其形成机制。结果表明:(1)两数据源分析得出的NO2浓度空间分布特征具有较好的一致性,苏南地区NO2浓度总体较高,柱状NO2浓度达到16.3 × 1015分子/cm 2,监测浓度达到46.3μg/m3,苏中地区NO2浓度相对较低,平均浓度为6 × 1015分子/cm 2, 26μg/m3。(2)宏观空间尺度下,苏南地区NO2柱平均浓度比苏北地区高9 × 1015分子/cm 2,监测浓度为15μg/m3;温度等自然因素是影响该尺度下NO2浓度分布不均一性的重要因素。(3)微观空间尺度上,苏南工业集中区、苏北部分供热城市和苏北工业园区NO2浓度高5 ~ 10%;NO2浓度随距离增大而逐渐降低;人口密度、GDP、汽车保有量等人为因素是影响该尺度下NO2浓度分布异质性的重要因素。基于以上发现,本文提出调整产业结构,限制高耗能、高排放企业数量,制定季节性减排措施。
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来源期刊
Resources Environment and Sustainability
Resources Environment and Sustainability Environmental Science-Environmental Science (miscellaneous)
CiteScore
15.10
自引率
0.00%
发文量
41
审稿时长
33 days
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