Deep learning for industrial processes: Forecasting amine emissions from a carbon capture plant

K. Jablonka, C. Charalambous, E. Sanchez Fernandez, G. Wiechers, P. Moser, Juliana Monteiro, B. Smit, S. Garcia
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Abstract

One of the main environmental impacts of amine-based carbon capture processes is the emission of the solvent and degradation products into the atmosphere. To mimic the mounting importance of intermittent operations of power plants we performed a stress test in which we measured the amine emissions from a pilot plant that has been in operation using a mixture of amines (CESAR1) in a slipstream from a coal-fired power plant. Understanding how changes in the operation far from the steady-state of the plant affect the emissions is key to designing emission mitigation strategies. However, conventional process modelling techniques struggle to capture the full dynamic, multivariate, and non-linear nature of this data. In this work, we report how a data-intensive approach can be used to learn the mapping between process and emissions from data. The resulting model can forecast the emissions, can be used to analyse the data and also perform in silico stress tests. By doing so, we reveal that emission mitigation strategies that work well for single component solvents (e.g. monoethanolamine) need to be revised for a mixture of solvents such as CESAR1. We expect that the combination of large amounts of data with flexible learning algorithms will impact the way we design and operate industrial processes, as we can now harvest information at conditions where conventional approaches fail.
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工业过程的深度学习:预测碳捕集厂的胺排放
胺基碳捕获工艺的主要环境影响之一是溶剂和降解产物排放到大气中。为了模拟发电厂间歇性运行的重要性,我们进行了一项压力测试,在该测试中,我们使用燃煤发电厂滑流中的胺混合物(CESAR1)测量了一个正在运行的中试装置的胺排放量。了解远离工厂稳态的运行变化如何影响排放是设计减排策略的关键。然而,传统的过程建模技术很难捕捉到这些数据的全部动态、多变量和非线性性质。在这项工作中,我们报告了如何使用数据密集型方法从数据中学习过程和排放之间的映射。由此产生的模型可以预测排放量,可以用于分析数据,也可以进行计算机应力测试。通过这样做,我们发现,对于单组分溶剂(如单乙醇胺)有效的减排策略需要针对混合溶剂(如CESAR1)进行修订。我们预计,大量数据与灵活的学习算法的结合将影响我们设计和操作工业流程的方式,因为我们现在可以在传统方法失败的情况下获取信息。
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