Small-angle scattering tensor tomography algorithm for robust reconstruction of complex textures.

IF 1.9 4区 材料科学 Q3 CHEMISTRY, MULTIDISCIPLINARY Acta Crystallographica Section A: Foundations and Advances Pub Date : 2023-11-01 Epub Date: 2023-10-19 DOI:10.1107/S205327332300863X
Leonard C Nielsen, Paul Erhart, Manuel Guizar-Sicairos, Marianne Liebi
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Abstract

The development of small-angle scattering tensor tomography has enabled the study of anisotropic nanostructures in a volume-resolved manner. It is of great value to have reconstruction methods that can handle many different nanostructural symmetries. For such a method to be employed by researchers from a wide range of backgrounds, it is crucial that its reliance on prior knowledge about the system is minimized, and that it is robust under various conditions. Here, a method is presented that employs band-limited spherical functions to enable the reconstruction of reciprocal-space maps of a wide variety of nanostructures. This method has been thoroughly tested and compared with existing methods in its ability to retrieve known reciprocal-space maps, as well as its robustness to changes in initial conditions, using both simulations and experimental data. It has also been evaluated for its computational performance. The anchoring of this method in a framework of integral geometry and linear algebra highlights its possibilities and limitations.

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用于复杂纹理鲁棒重建的小角度散射张量层析成像算法。
小角度散射张量层析成像的发展使各向异性纳米结构的研究成为可能。拥有能够处理许多不同纳米结构对称性的重建方法是非常有价值的。对于来自各种背景的研究人员使用这种方法,至关重要的是,它要最大限度地减少对系统先验知识的依赖,并且在各种条件下都是稳健的。在此,提出了一种方法,该方法使用带限球形函数来重建各种纳米结构的倒数空间图。使用模拟和实验数据,该方法在检索已知倒数空间图的能力以及对初始条件变化的鲁棒性方面已经与现有方法进行了彻底的测试和比较。它的计算性能也得到了评估。这种方法在积分几何和线性代数框架中的锚定突出了它的可能性和局限性。
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来源期刊
Acta Crystallographica Section A: Foundations and Advances
Acta Crystallographica Section A: Foundations and Advances CHEMISTRY, MULTIDISCIPLINARYCRYSTALLOGRAPH-CRYSTALLOGRAPHY
CiteScore
2.60
自引率
11.10%
发文量
419
期刊介绍: Acta Crystallographica Section A: Foundations and Advances publishes articles reporting advances in the theory and practice of all areas of crystallography in the broadest sense. As well as traditional crystallography, this includes nanocrystals, metacrystals, amorphous materials, quasicrystals, synchrotron and XFEL studies, coherent scattering, diffraction imaging, time-resolved studies and the structure of strain and defects in materials. The journal has two parts, a rapid-publication Advances section and the traditional Foundations section. Articles for the Advances section are of particularly high value and impact. They receive expedited treatment and may be highlighted by an accompanying scientific commentary article and a press release. Further details are given in the November 2013 Editorial. The central themes of the journal are, on the one hand, experimental and theoretical studies of the properties and arrangements of atoms, ions and molecules in condensed matter, periodic, quasiperiodic or amorphous, ideal or real, and, on the other, the theoretical and experimental aspects of the various methods to determine these properties and arrangements.
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