Thermal physical applications of carbon dioxide: Recent progress, challenges and perspective

Pei Duan, Kun Jiang, Jinwen Shi, Hui Jin
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Abstract

Carbon dioxide (CO2) is one of the main factors contributing to the greenhouse effect. The dependence on fossil fuels has led to increasing levels of carbon dioxide in the atmosphere every year. And it is far from enough to solve the climate problem by reducing the consumption of fossil fuels to cut down carbon dioxide emissions. In recent years, a series of researches on Carbon Capture, Utilization and Storage (CCUS) have been carried out in various countries around the world. CO2 is a nontoxic, tasteless and stable gas at normal temperature. However, when it reaches supercritical state after rising temperature and pressure, it has the characteristics of low viscosity, high diffusivity and high density, and is widely used in green, pollution-free and efficient development technology. Because of these unique properties, supercritical carbon dioxide (sCO2) has attracted more and more attention from researchers. sCO2 has been widely used in many aspects by virtue of its high solubility and easy compression. Different from previous reviews which only introduced the application of sCO2 property, this paper introduces the current research status of the application of the thermodynamic property of carbon dioxide in extraction, dyeing, pharmaceutical, power generation, heat transfer and exploitation of unconventional oil and gas, and mainly analyzes each application in detail from the aspects of working mechanism and improving working efficiency. Finally, the research direction and problems needed to be solved for the application of CO2 thermal physics are proposed, which pave the way for other new applications.

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二氧化碳的热物理应用:最新进展、挑战和展望
二氧化碳(CO2)是造成温室效应的主要因素之一。对化石燃料的依赖导致大气中的二氧化碳含量每年都在增加。仅仅通过减少化石燃料的消耗来减少二氧化碳排放来解决气候问题是远远不够的。近年来,世界各国对碳捕获、利用和储存(CCUS)进行了一系列研究。二氧化碳在常温下是一种无毒、无味、稳定的气体。然而,当它在升温升压后达到超临界状态时,它具有低粘度、高扩散率和高密度的特点,被广泛应用于绿色、无污染、高效的开发技术中。由于这些独特的性质,超临界二氧化碳(sCO2)越来越受到研究人员的关注。sCO2以其高溶解性和易压缩性在许多方面得到了广泛的应用。与以往仅介绍sCO2性质应用的综述不同,本文介绍了二氧化碳热力学性质在萃取、染色、制药、发电、传热和非常规油气开发中的应用研究现状,并主要从工作机制和提高工作效率两个方面对每种应用进行了详细的分析。最后,提出了CO2热物理应用的研究方向和需要解决的问题,为其他新的应用铺平了道路。
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Outside Front Cover Table of Contents Outside Back Cover On controllability of fluidized bed reduction of iron ore by CH4 for selective formation of magnetite Organics-based Aqueous Batteries: Concept for Stationary Energy Storage with Resource Feasibility
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