Utilization of compressed natural gas for the production of carbon nanotubes

Kim-Yang Lee , Wei-Ming Yeoh , Siang-Piao Chai , Abdul Rahman Mohamed
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引用次数: 6

Abstract

The present work aims at utilizing compressed natural gas (CNG) as carbon source for the synthesis of carbon nanotubes (CNTs) over CoO-MoO/Al2O3 catalyst via catalytic chemical vapor deposition (CCVD) method. The as-produced carbonaceous product was characterized by thermal gravimetric analyzer (TGA), scanning electron microscopy (SEM), transmission electron microscopy (TEM) and Raman spectroscopy. The experimental finding shows that CNTs were successfully produced from CNG while carbon nanofibers (CNFs) were formed as the side products. In addition, the catalytic activity and lifetime were found sustained and prolonged, as compared with using high purity methane as carbon source. The present study suggests an alternative route which can effectively produce CNTs and CNFs using low cost CNG.

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利用压缩天然气生产碳纳米管
本研究旨在利用压缩天然气(CNG)作为碳源,通过催化化学气相沉积(CCVD)方法在co - moo /Al2O3催化剂上合成碳纳米管(CNTs)。采用热重分析仪(TGA)、扫描电子显微镜(SEM)、透射电子显微镜(TEM)和拉曼光谱对产物进行了表征。实验结果表明,CNG成功制备了碳纳米管,同时作为副产物形成了碳纳米纤维。此外,与使用高纯甲烷作为碳源相比,其催化活性和寿命持续延长。本研究提出了一种利用低成本CNG有效生产碳纳米管和cnf的替代途径。
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来源期刊
Journal of Natural Gas Chemistry
Journal of Natural Gas Chemistry 化学-工程:化工
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2 months
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