Possible Ground States and Magnetic-Field-Tuned Phase Transitions of a Geometrically Frustrated Ising Antiferromagnet on a Triangular Lattice

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2023-03-08 DOI:10.1109/LMAG.2023.3274049
Thao Huong Pham
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Abstract

Possible average alignments of the spins in the ground state and the phase transitions of a geometrically frustrated Ising antiferromagnet in the presence of magnetic fields on a triangular lattice are studied in a mean field approximation. Starting from a zero-field clock phase, we can determine the phase boundaries from the curves of magnetic moments and their derivatives as functions of the fields. We also analyze the behavior of sublattice magnetic moments under the effect of the fields. The experimental relevances for TmMgGaO 4 and SrEr 2 O 4 are discussed. Besides, using a functional integral method, we have calculated a functional for free energy to obtain the contribution of spin fluctuations. From this, we can find that the role of the quantum spin fluctuations at very low temperatures is only prominent in the vicinity of the transition points. It can therefore be seen that the results, although given in the mean field approximation, describe quite well the phase transitions and rearrangements of the magnetic moment per spin under the effect of both the transverse and longitudinal fields.
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三角晶格上几何抑制的Ising反铁磁体的可能基态和磁场调谐相变
在平均场近似下,研究了在三角形晶格上存在磁场的情况下,几何受抑的伊辛反铁磁体基态自旋的可能平均排列和相变。从零场时钟相位开始,我们可以根据磁矩及其导数作为场函数的曲线来确定相位边界。我们还分析了场作用下亚晶格磁矩的行为。讨论了TmMgGaO4和SrEr2O4的实验相关性。此外,利用泛函积分方法,我们计算了自由能的泛函,得到了自旋涨落的贡献。由此,我们可以发现,在非常低的温度下,量子自旋涨落的作用只在跃迁点附近突出。因此可以看出,尽管这些结果是在平均场近似中给出的,但它们很好地描述了在横向场和纵向场的影响下每自旋磁矩的相变和重排。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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