{"title":"Possible Ground States and Magnetic-Field-Tuned Phase Transitions of a Geometrically Frustrated Ising Antiferromagnet on a Triangular Lattice","authors":"Thao Huong Pham","doi":"10.1109/LMAG.2023.3274049","DOIUrl":null,"url":null,"abstract":"Possible average alignments of the spins in the ground state and the phase transitions of a geometrically frustrated Ising antiferromagnet in the presence of magnetic fields on a triangular lattice are studied in a mean field approximation. Starting from a zero-field clock phase, we can determine the phase boundaries from the curves of magnetic moments and their derivatives as functions of the fields. We also analyze the behavior of sublattice magnetic moments under the effect of the fields. The experimental relevances for TmMgGaO\n<sub>4</sub>\n and SrEr\n<sub>2</sub>\nO\n<sub>4</sub>\n are discussed. Besides, using a functional integral method, we have calculated a functional for free energy to obtain the contribution of spin fluctuations. From this, we can find that the role of the quantum spin fluctuations at very low temperatures is only prominent in the vicinity of the transition points. It can therefore be seen that the results, although given in the mean field approximation, describe quite well the phase transitions and rearrangements of the magnetic moment per spin under the effect of both the transverse and longitudinal fields.","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2023-03-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"101","ListUrlMain":"https://ieeexplore.ieee.org/document/10120918/","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Possible average alignments of the spins in the ground state and the phase transitions of a geometrically frustrated Ising antiferromagnet in the presence of magnetic fields on a triangular lattice are studied in a mean field approximation. Starting from a zero-field clock phase, we can determine the phase boundaries from the curves of magnetic moments and their derivatives as functions of the fields. We also analyze the behavior of sublattice magnetic moments under the effect of the fields. The experimental relevances for TmMgGaO
4
and SrEr
2
O
4
are discussed. Besides, using a functional integral method, we have calculated a functional for free energy to obtain the contribution of spin fluctuations. From this, we can find that the role of the quantum spin fluctuations at very low temperatures is only prominent in the vicinity of the transition points. It can therefore be seen that the results, although given in the mean field approximation, describe quite well the phase transitions and rearrangements of the magnetic moment per spin under the effect of both the transverse and longitudinal fields.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.