Uncertainty evaluation in activity measurements with HPGe using two relative methods

M. C. M. De Almeida, J. U. Delgado, R. L. Silva, R. Poledna, R. S. Gomes, A. L. Ferreira Filho
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Abstract

Radionuclide metrology laboratories aim to provide radioactive standards for detector calibrations in nuclear safety areas with low uncertainties.  Such standards are applied in nuclear industries, according to the requirements of monitoring programmes. The standard radionuclides of 133Ba, 152Eu and 166mHo are suitable to the determination of efficiency curves in HPGe detectors due to their multi-gamma emissions, which are intense and well separate in the spectrum. With efficiency curves it is possible to do the measurements without needing to use standards. In this work was made a verifying of the uncertainties obtained for the two relative methods: comparative (sample-standard) and efficiency curve. The total uncertainties obtained by sample-standard method varied from 0.4 to 1.2 % (k=1). The results using efficiency curve method are between 0.9 to 2.2 % (k=1).
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用两种相对方法评价HPGe活度测量中的不确定度
放射性核素计量实验室旨在为核安全领域的探测器校准提供低不确定度的放射性标准。根据监测方案的要求,这些标准适用于核工业。133Ba、152Eu和166mHo三种标准放射性核素的多伽马辐射强度强,光谱分离性好,适合测定HPGe探测器的效率曲线。有了效率曲线,就可以在不使用标准的情况下进行测量。本文对比较法(样品-标准法)和效率曲线法两种相对方法的不确定度进行了验证。样品-标准法测定的总不确定度为0.4 ~ 1.2% (k=1)。效率曲线法测定结果在0.9 ~ 2.2%之间(k=1)。
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