Analysis of the temporal variability of CO2, CH4 and CO concentrations at Lamto, West Africa

Toure Dro Tiemoko, M. Ramonet, Fidèle Yoroba, K. B. Kouassi, K. Kouadio, V. Kazan, C. Kaiser, F. Truong, C. Vuillemin, M. Delmotte, B. Wastine, P. Ciais
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引用次数: 7

Abstract

Abstract The 10-year observations of the atmospheric molar fractions of CO2, CH4 and CO in West Africa were analyzed using a high precision measurement of the Lamto (LTO) station (6°31 N and 5°02 W) in Côte d’Ivoire. At daily scale, high concentrations appear at night with significant peaks around 7 a.m. local time and minimum concentrations in the afternoon for CO2 and CH4. The CO concentrations show two peaks around 8 h and 20 h corresponding to the maximum in road traffic of a northern motorway located 14 km from the station. The long-term increase rates of CH4 (∼7 ppb year−1) and CO2 (∼2.24 ppm year−1) at Lamto are very close to global trends. The variations of the concentrations of the three gases show strong seasonality with a peak in January for all gases and minima in September for CO2 and CH4, and in June for CO. The CO variation suggests a significant impact of fires on the CO, CO2 and CH4 anomalies in the Lamto region during the dry season (December to February). CO and CH4 show strong correlations (at synoptic-scale and monthly based) in January (r = 0.84), February (r = 0.90), April (r = 0.74), November (r = 0.79) and December (r = 0.72) reflecting similar sources of emission for both gases. The trajectories of polluted air masses at LTO, also indicate continental sources of emission associated with Harmattan winds.
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西非Lamto地区CO2、CH4和CO浓度的时间变异分析
摘要利用位于Côte科特迪瓦的Lamto (LTO)站(6°31 N和5°02 W)的高精度测量数据,分析了西非地区10年大气CO2、CH4和CO的摩尔分数。在日尺度上,CO2和CH4的高浓度出现在夜间,在当地时间早上7点左右达到峰值,下午浓度最低。CO浓度在8 h和20 h出现两个峰值,对应于距离站点14 km的北部高速公路的道路交通最大值。Lamto的CH4 (~ 7 ppb - 1年)和CO2 (~ 2.24 ppm - 1年)的长期增长率非常接近全球趋势。3种气体的浓度变化均表现出较强的季节性,其中CO2和CH4在1月达到峰值,CO2和CH4在9月达到最低点,CO在6月达到最低点。CO的变化表明,12月至2月枯水期林火对Lamto地区CO、CO2和CH4异常有显著影响。CO和CH4在1月(r = 0.84)、2月(r = 0.90)、4月(r = 0.74)、11月(r = 0.79)和12月(r = 0.72)表现出较强的相关性(在天气尺度和月基础上),反映出两种气体的排放源相似。LTO受污染气团的轨迹也显示了与哈马丹风有关的大陆排放源。
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