Determination of Naturally Occurring Radionuclides Concentration in Environmental Samples in West Kirby Area Using Gamma-Ray Spectroscopy

Ekundayo Oki Akinduro
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Abstract

The purpose of this work is to investigate and evaluate the level of contamination of naturally occurring radionuclides in environmental soil samples collected at a place from West Kirby using gamma-ray spectroscopy. The Broad Energy Germanium (BEGe2825) detector has the ability to detect gamma-rays in the range of 3 keV-3MeV. This detector offers a very good resolution, low noise performance and almost ideal Gaussian shape in our analysis. Under our depth of interest of 0 – 48 cm, a total of six spectra were measured. From known values of gamma-ray energies, a calibrated curve was plotted. From the analysis, the mean activity concentration of naturally radionuclides of uranium-238, thorium-232 and potassium-40 obtained are 6.7 ± 0.1 Bq/kg, 5.6 ± 0.1Bq/kg and 398.2± 8.2 Bq/kg were found in the range of (5.37 ± 0.30- 8.86 ±0.40) Bq/kg, (4.37 ± 0.31- 8.72 ±0.35) Bq/kg and (384 ± 19 and 416 ± 21) Bq/kg respectively. Man-made radionuclides of americium-241 and cesium-137 mean activity concentrations are 4.3± 0.1 Bq/kg and 14.5 ± 0.3 Bq/kg were found in the range of (BDL: 5.95±0.32) Bq/kg and (6.66 ± 0.35- 29.2 ±1.5) Bq/kg respectively.
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伽玛射线光谱法测定西柯比地区环境样品中自然存在的放射性核素浓度
这项工作的目的是调查和评估在西柯比一个地方收集的环境土壤样本中天然存在的放射性核素的污染水平,使用伽马射线光谱。宽能锗(BEGe2825)探测器能够探测3k - 3mev范围内的伽马射线。在我们的分析中,该检测器提供了非常好的分辨率,低噪声性能和几乎理想的高斯形状。在我们的兴趣深度0 - 48 cm下,总共测量了6个光谱。根据已知的伽马射线能量值,绘制了校准曲线。分析得到的天然放射性核素铀-238、钍-232和钾-40的平均活度浓度分别为6.7±0.1Bq/kg、5.6±0.1Bq/kg和398.2±8.2 Bq/kg,范围分别为(5.37±0.30 ~ 8.86±0.40)Bq/kg、(4.37±0.31 ~ 8.72±0.35)Bq/kg和(384±19和416±21)Bq/kg。人造放射性核素镅-241和铯-137的平均活度浓度分别为(5.95±0.32)Bq/kg和(6.66±0.35 ~ 29.2±1.5)Bq/kg,平均活度浓度分别为4.3±0.1 Bq/kg和14.5±0.3 Bq/kg。
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