Domain Structure in Ferroelectric Thin Films

N. Yunga, A. M. Dikandé
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Abstract

At low temperatures, uniaxial perovskites exhibit a spontaneous polarization with a permanent dipole moment. The broken symmetry state involves an order parameter and dielectric properties of the materials which are strongly dominated by a one-dimensional physics. For the last sixty years there has been growing interest in these crystals for potential applications in communication technology. Very recently, renewed interest to ferroelectric memory devices has been remarkable with particular emphasis on miniaturized devices. This new perspective comes along with great challenges, one of which is the critical size for stable domains in thin ferroelectric crystals. Since the polarization switching involves a pre-existing spontaneous polarization, it is of fundamental importance to address the question of conditions under which polarized domains can develop in a ferroelectric thin film. From previous articles, it has been observed that most studies focus on numerical simulations which is a good approach but for the fact that numerical simulations involve approximation of physical quantities, which is limitation to comparing experimental with theoretical studies. This motivated the authors to look purely at an analytical approach taking advantage of the new mathematical approach in the study of nonlinear systems. In this work, the authors have considered the question from an analytical point of view, focusing on an interesting model introduced by Lu and Cao. We propose an analytical counterpart of the numerical simulations done in this previous study.
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铁电薄膜中的畴结构
在低温下,单轴钙钛矿表现出具有永久偶极矩的自发极化。对称性破缺态涉及到材料的序参量和介电性质,它们受一维物理的强烈支配。在过去的60年里,人们对这些晶体在通信技术中的潜在应用越来越感兴趣。最近,人们对铁电存储器件重新产生了兴趣,特别是小型化器件。这一新观点带来了巨大的挑战,其中之一是薄铁电晶体中稳定畴的临界尺寸。由于极化开关涉及预先存在的自发极化,因此解决铁电薄膜中极化域形成的条件问题具有重要的基础意义。从以前的文章中可以看出,大多数研究都集中在数值模拟上,这是一种很好的方法,但是数值模拟涉及到物理量的近似,这限制了实验研究与理论研究的比较。这促使作者纯粹着眼于分析方法,利用新的数学方法来研究非线性系统。在本书中,作者从分析的角度考虑了这个问题,重点关注了卢和曹介绍的一个有趣的模型。我们提出了一种与先前研究中所做的数值模拟相对应的分析方法。
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