Xianda Gong, Jiaoshi Zhang, Betty Croft, Xin Yang, Markus M. Frey, Nora Bergner, Rachel Y.-W. Chang, Jessie M. Creamean, Chongai Kuang, Randall V. Martin, Ananth Ranjithkumar, Arthur J. Sedlacek, Janek Uin, Sascha Willmes, Maria A. Zawadowicz, Jeffrey R. Pierce, Matthew D. Shupe, Julia Schmale, Jian Wang
{"title":"吹雪产生的大量细海盐气溶胶导致北极变暖","authors":"Xianda Gong, Jiaoshi Zhang, Betty Croft, Xin Yang, Markus M. Frey, Nora Bergner, Rachel Y.-W. Chang, Jessie M. Creamean, Chongai Kuang, Randall V. Martin, Ananth Ranjithkumar, Arthur J. Sedlacek, Janek Uin, Sascha Willmes, Maria A. Zawadowicz, Jeffrey R. Pierce, Matthew D. Shupe, Julia Schmale, Jian Wang","doi":"10.1038/s41561-023-01254-8","DOIUrl":null,"url":null,"abstract":"The Arctic warms nearly four times faster than the global average, and aerosols play an increasingly important role in Arctic climate change. In the Arctic, sea salt is a major aerosol component in terms of mass concentration during winter and spring. However, the mechanisms of sea salt aerosol production remain unclear. Sea salt aerosols are typically thought to be relatively large in size but low in number concentration, implying that their influence on cloud condensation nuclei population and cloud properties is generally minor. Here we present observational evidence of abundant sea salt aerosol production from blowing snow in the central Arctic. Blowing snow was observed more than 20% of the time from November to April. The sublimation of blowing snow generates high concentrations of fine-mode sea salt aerosol (diameter below 300 nm), enhancing cloud condensation nuclei concentrations up to tenfold above background levels. Using a global chemical transport model, we estimate that from November to April north of 70° N, sea salt aerosol produced from blowing snow accounts for about 27.6% of the total particle number, and the sea salt aerosol increases the longwave emissivity of clouds, leading to a calculated surface warming of +2.30 W m−2 under cloudy sky conditions. Fine sea salt aerosols produced by blowing snow in the Arctic impact cloud properties and warm the surface, according to observations from the MOSAiC expedition.","PeriodicalId":19053,"journal":{"name":"Nature Geoscience","volume":"16 9","pages":"768-774"},"PeriodicalIF":15.7000,"publicationDate":"2023-09-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10482690/pdf/","citationCount":"2","resultStr":"{\"title\":\"Arctic warming by abundant fine sea salt aerosols from blowing snow\",\"authors\":\"Xianda Gong, Jiaoshi Zhang, Betty Croft, Xin Yang, Markus M. Frey, Nora Bergner, Rachel Y.-W. Chang, Jessie M. Creamean, Chongai Kuang, Randall V. Martin, Ananth Ranjithkumar, Arthur J. Sedlacek, Janek Uin, Sascha Willmes, Maria A. Zawadowicz, Jeffrey R. Pierce, Matthew D. Shupe, Julia Schmale, Jian Wang\",\"doi\":\"10.1038/s41561-023-01254-8\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The Arctic warms nearly four times faster than the global average, and aerosols play an increasingly important role in Arctic climate change. In the Arctic, sea salt is a major aerosol component in terms of mass concentration during winter and spring. However, the mechanisms of sea salt aerosol production remain unclear. Sea salt aerosols are typically thought to be relatively large in size but low in number concentration, implying that their influence on cloud condensation nuclei population and cloud properties is generally minor. Here we present observational evidence of abundant sea salt aerosol production from blowing snow in the central Arctic. Blowing snow was observed more than 20% of the time from November to April. The sublimation of blowing snow generates high concentrations of fine-mode sea salt aerosol (diameter below 300 nm), enhancing cloud condensation nuclei concentrations up to tenfold above background levels. Using a global chemical transport model, we estimate that from November to April north of 70° N, sea salt aerosol produced from blowing snow accounts for about 27.6% of the total particle number, and the sea salt aerosol increases the longwave emissivity of clouds, leading to a calculated surface warming of +2.30 W m−2 under cloudy sky conditions. Fine sea salt aerosols produced by blowing snow in the Arctic impact cloud properties and warm the surface, according to observations from the MOSAiC expedition.\",\"PeriodicalId\":19053,\"journal\":{\"name\":\"Nature Geoscience\",\"volume\":\"16 9\",\"pages\":\"768-774\"},\"PeriodicalIF\":15.7000,\"publicationDate\":\"2023-09-04\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10482690/pdf/\",\"citationCount\":\"2\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nature Geoscience\",\"FirstCategoryId\":\"89\",\"ListUrlMain\":\"https://www.nature.com/articles/s41561-023-01254-8\",\"RegionNum\":1,\"RegionCategory\":\"地球科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"GEOSCIENCES, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nature Geoscience","FirstCategoryId":"89","ListUrlMain":"https://www.nature.com/articles/s41561-023-01254-8","RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"GEOSCIENCES, MULTIDISCIPLINARY","Score":null,"Total":0}
Arctic warming by abundant fine sea salt aerosols from blowing snow
The Arctic warms nearly four times faster than the global average, and aerosols play an increasingly important role in Arctic climate change. In the Arctic, sea salt is a major aerosol component in terms of mass concentration during winter and spring. However, the mechanisms of sea salt aerosol production remain unclear. Sea salt aerosols are typically thought to be relatively large in size but low in number concentration, implying that their influence on cloud condensation nuclei population and cloud properties is generally minor. Here we present observational evidence of abundant sea salt aerosol production from blowing snow in the central Arctic. Blowing snow was observed more than 20% of the time from November to April. The sublimation of blowing snow generates high concentrations of fine-mode sea salt aerosol (diameter below 300 nm), enhancing cloud condensation nuclei concentrations up to tenfold above background levels. Using a global chemical transport model, we estimate that from November to April north of 70° N, sea salt aerosol produced from blowing snow accounts for about 27.6% of the total particle number, and the sea salt aerosol increases the longwave emissivity of clouds, leading to a calculated surface warming of +2.30 W m−2 under cloudy sky conditions. Fine sea salt aerosols produced by blowing snow in the Arctic impact cloud properties and warm the surface, according to observations from the MOSAiC expedition.
期刊介绍:
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