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Author Correction: Oxygen priming induced by elevated CO2 reduces carbon accumulation and methane emissions in coastal wetlands 作者更正:高浓度二氧化碳诱导的引氧减少了沿海湿地的碳积累和甲烷排放
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-22 DOI: 10.1038/s41561-024-01611-1
Genevieve L. Noyce, Alexander J. Smith, Matthew L. Kirwan, Roy L. Rich, J. Patrick Megonigal

Correction to: Nature Geoscience https://doi.org/10.1038/s41561-022-01070-6, published online 5 January 2023.

更正为自然-地球科学》https://doi.org/10.1038/s41561-022-01070-6,2023 年 1 月 5 日在线发表。
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引用次数: 0
Multi-month forecasts of marine heatwaves and ocean acidification extremes 海洋热浪和海洋酸化极端事件的多月预报
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-21 DOI: 10.1038/s41561-024-01593-0
Samuel C. Mogen, Nicole S. Lovenduski, Stephen G. Yeager, Antonietta Capotondi, Michael G. Jacox, Stephen Bograd, Emanuele Di Lorenzo, Elliot L. Hazen, Mercedes Pozo Buil, Who Kim, Nan Rosenbloom

Marine heatwaves and ocean acidification extreme events are periods during which temperature and acidification reach statistically extreme levels (90th percentile), relative to normal variability, potentially endangering ecosystems. As the threats from marine heatwaves and ocean acidification extreme events grow with climate change, there is need for skilful predictions of events months to years in advance. Previous work has demonstrated that climate models can predict marine heatwaves up to 12 months in advance in key regions, but forecasting of ocean acidification extreme events has been difficult due to the complexity of the processes leading to extremes and sparse observations. Here we use the Community Earth System Model Seasonal-to-Multiyear Large Ensemble to make predictions of marine heatwaves and two forms of ocean acidification extreme events, as defined by anomalies in hydrogen ion concentration and aragonite saturation state. We show that the ensemble skilfully predicts marine heatwaves and ocean acidification extreme events as defined by aragonite saturation state up to 1 year in advance. Predictive skill for ocean acidification extremes as defined by hydrogen ion concentration is lower, probably reflecting mismatch between model and observed state. Skill is highest in the eastern Pacific, reflecting the predictable contribution of El Niño/Southern Oscillation to regional variability. A forecast generated in late 2023 during the 2023–2024 El Niño event finds high likelihood for widespread marine heatwaves and ocean acidification extreme events in 2024.

海洋热浪和海洋酸化极端事件是指相对于正常变化而言,温度和酸化达到统计意义上的极端水平(第 90 百分位数),可能危及生态系统的时期。随着气候变化,海洋热浪和海洋酸化极端事件的威胁也越来越大,因此需要提前数月至数年对事件进行娴熟的预测。以往的工作表明,气候模式可以提前 12 个月预测主要地区的海洋热浪,但由于导致极端事件的过程复杂且观测稀少,海洋酸化极端事件的预测一直很困难。在这里,我们利用群落地球系统模式季节-多年大型集合来预测海洋热浪和两种形式的海洋酸化极端事件,这两种极端事件是由氢离子浓度和文石饱和状态的异常所定义的。我们的研究表明,该集合可提前一年娴熟地预测海洋热浪和以霰石饱和状态定义的海洋酸化极端事件。对以氢离子浓度定义的海洋酸化极端事件的预测能力较低,这可能反映了模式与观测状态之间的不匹配。东太平洋的预测技能最高,反映了厄尔尼诺/南方涛动对区域变化的可预测性。在 2023-2024 年厄尔尼诺现象期间于 2023 年底生成的预测发现,2024 年发生大范围海洋热浪和海洋酸化极端事件的可能性很高。
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引用次数: 0
Arctic freshwater anomaly transiting to the North Atlantic delayed within a buffer zone 在缓冲区内延迟向北大西洋传输的北极淡水异常点
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-20 DOI: 10.1038/s41561-024-01592-1
Qiang Wang, Sergey Danilov, Thomas Jung

A two-decade-long accumulation of freshwater in the Arctic Ocean’s Beaufort Gyre has recently started to be released. Here we use satellite observations and model simulations to show that changes in wind regimes and sea ice declines are causing freshwater to accumulate close to the export gateways to the North Atlantic. This emerging buffer zone plays an important role in modulating the propagation of freshwater into the subpolar North Atlantic.

北冰洋波弗特环流中长达二十年的淡水积累最近开始释放。在这里,我们利用卫星观测数据和模型模拟结果表明,风向的变化和海冰的减少正在导致淡水在北大西洋出口门户附近积聚。这个新出现的缓冲区在调节淡水向北大西洋副极地的传播方面发挥着重要作用。
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引用次数: 0
Low-elevation forest extent in the western United States constrained by soil surface temperatures 受土壤表面温度制约的美国西部低海拔森林范围
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-19 DOI: 10.1038/s41561-024-01577-0
Zachary A. Holden, Solomon Z. Dobrowski, Alan Swanson, Zachary Hoylman, Drew Lyons, Allen Warren, Marco Maneta

Climate change and disturbance threaten forested ecosystems across the globe. Our ability to predict the future distribution of forests requires understanding the limiting factors for regeneration. Forest canopies buffer against near-surface air temperature and vapour pressure deficit extremes, and ongoing losses of forest canopy from disturbances such as wildfire can exacerbate climate constraints on natural regeneration. Here we combine experimental, empirical and simulation-based evidence to show that soil surface temperatures constrain the low-elevation extent of forests in the western United States. Simulated potential soil surface temperatures predict the position of the low-elevation forest treeline, exhibiting temperature thresholds consistent with field and laboratory studies. High-resolution historical and future surface temperature maps show that 107,000–238,000 km2 (13–20%) of currently forested area exceeds the critical thermal threshold for forest regeneration and this area is projected to more than double by 2050. Soil surface temperature is an important physical control on seedling survival at low elevations that will likely be an increasing constraint on the extent of western United States forests as the climate warms.

气候变化和干扰威胁着全球的森林生态系统。我们要想预测森林未来的分布,就必须了解再生的限制因素。森林树冠可以缓冲近地表的极端气温和蒸汽压力不足,野火等干扰造成的森林树冠持续损失会加剧气候对自然再生的限制。在这里,我们结合实验、经验和模拟证据,证明土壤表面温度制约着美国西部森林的低海拔范围。模拟的潜在土壤表面温度预测了低海拔森林树线的位置,显示出与野外和实验室研究一致的温度阈值。高分辨率的历史和未来地表温度地图显示,目前有 107,000-238,000 平方公里(13-20%)的森林面积超过了森林再生的临界温度阈值,预计到 2050 年这一面积将增加一倍以上。土壤表面温度是低海拔地区幼苗存活的一个重要物理控制因素,随着气候变暖,这可能会对美国西部森林的范围造成越来越大的限制。
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引用次数: 0
Weakening of the Atlantic Meridional Overturning Circulation driven by subarctic freshening since the mid-twentieth century 二十世纪中叶以来亚北极清新驱动的大西洋经向翻转环流减弱现象
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-18 DOI: 10.1038/s41561-024-01568-1
Gabriel M. Pontes, Laurie Menviel

The Atlantic Meridional Overturning Circulation is the main driver of northward heat transport in the Atlantic Ocean today, setting global climate patterns. Whether global warming has affected the strength of this overturning circulation over the past century is still debated: observational studies suggest that there has been persistent weakening since the mid-twentieth century, whereas climate models systematically simulate a stable circulation. Here, using Earth system and eddy-permitting coupled ocean–sea-ice models, we show that a freshening of the subarctic Atlantic Ocean and weakening of the overturning circulation increase the temperature and salinity of the South Atlantic on a decadal timescale through the propagation of Kelvin and Rossby waves. We also show that accounting for upper-end meltwater input in historical simulations significantly improves the data–model agreement on past changes in the Atlantic Meridional Overturning Circulation, yielding a slowdown of 0.46 sverdrups per decade since 1950. Including estimates of subarctic meltwater input for the coming century suggests that this circulation could be 33% weaker than its anthropogenically unperturbed state under 2 °C of global warming, which could be reached over the coming decade. Such a weakening of the overturning circulation would substantially affect the climate and ecosystems.

大西洋经向翻转环流是当今大西洋热量向北输送的主要驱动力,决定着全球气候模式。在过去的一个世纪中,全球变暖是否影响了这一翻转环流的强度仍存在争议:观测研究表明,自二十世纪中叶以来,这一环流持续减弱,而气候模式则系统地模拟了稳定的环流。在这里,我们利用地球系统和允许涡流的海洋-海冰耦合模式表明,亚北极大西洋的清新和翻转环流的减弱通过开尔文波和罗斯比波的传播,在十年时间尺度上增加了南大西洋的温度和盐度。我们还表明,在历史模拟中考虑上端融水输入可显著改善大西洋经向翻转环流过去变化的数据-模型一致性,自 1950 年以来每十年减慢 0.46 sverdrups。根据对未来一个世纪亚北极融水输入的估计,在全球变暖 2 ℃ 的情况下,这一环流可能会比其人为未扰动状态减弱 33%。这种翻转环流的减弱将对气候和生态系统产生重大影响。
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引用次数: 0
Recovery of ecosystem productivity in China due to the Clean Air Action plan 中国因清洁空气行动计划而恢复生态系统生产力
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-15 DOI: 10.1038/s41561-024-01586-z
Hao Zhou, Xu Yue, Huibin Dai, Guannan Geng, Wenping Yuan, Jiquan Chen, Guofeng Shen, Tianyi Zhang, Jun Zhu, Hong Liao

Severe air pollution reduces ecosystem carbon assimilation through the vegetation damaging effects of ozone and by altering the climate through aerosol effects, exacerbating global warming. In response, China implemented the Clean Air Action plan in 2013 to reduce anthropogenic emissions. Here we assess the impact of air pollution reductions due to the Clean Air Action plan on net primary productivity (NPP) in China during the period 2014–2020 using multiple measurements, process-based models and machine learning algorithms. The Clean Air Action plan led to a national NPP increase of 26.3 ± 27.9 TgC yr−1, of which 20.1 ± 10.9 TgC yr−1 is attributed to aerosol reductions, driven by both the enhanced light availability as a result of decreased black carbon concentrations and the increased precipitation caused by weakened aerosol climatic effects. The impact of ozone amelioration became more important over time, surpassing the effects of aerosol reduction by 2020, and is expected to drive future NPP recovery. Two machine learning models simulated similar NPP recoveries of 42.8 ± 26.8 TgC yr1 and 43.4 ± 30.1 TgC yr1. Our study highlights substantial carbon gains from controlling aerosols and surface ozone, underscoring the co-benefits of regulating air pollution for public health and carbon neutrality in China.

严重的空气污染通过臭氧对植被的破坏作用,以及通过气溶胶效应改变气候来减少生态系统的碳同化,从而加剧全球变暖。为此,中国于 2013 年实施了 "清洁空气行动计划",以减少人为排放。在此,我们利用多种测量数据、基于过程的模型和机器学习算法,评估了 2014-2020 年间清洁空气行动计划导致的空气污染减排对中国净初级生产力(NPP)的影响。清洁空气行动计划使全国净初级生产力增加了 26.3 ± 27.9 TgC yr-1,其中 20.1 ± 10.9 TgC yr-1归因于气溶胶的减少,这既是由于黑碳浓度降低导致光照可用性增强,也是由于气溶胶气候效应减弱导致降水量增加。随着时间的推移,臭氧改善的影响变得越来越重要,到 2020 年将超过气溶胶减少的影响,预计将推动未来 NPP 的恢复。两个机器学习模型模拟的净生产力恢复量相似,分别为 42.8 ± 26.8 TgC yr-1 和 43.4 ± 30.1 TgC yr-1。我们的研究突显了控制气溶胶和地表臭氧所带来的巨大碳收益,强调了在中国控制空气污染对公众健康和碳中和的共同效益。
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引用次数: 0
Coupled decline in ocean pH and carbonate saturation during the Palaeocene–Eocene Thermal Maximum 古新世-始新世热极盛期海洋 pH 值和碳酸盐饱和度的耦合下降
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-12 DOI: 10.1038/s41561-024-01579-y
Mingsong Li, Lee R. Kump, Andy Ridgwell, Jessica E. Tierney, Gregory J. Hakim, Steven B. Malevich, Christopher J. Poulsen, Robert Tardif, Haoxun Zhang, Jiang Zhu

The Palaeocene–Eocene Thermal Maximum, a climate event 56 million years ago, was characterized by rapid carbon release and extensive ocean acidification. However, our understanding of acidification and the evolution of ocean saturation states continues to be hindered by considerable uncertainties, primarily stemming from the limited availability of proxy data. Under such conditions, data assimilation allows for an internally consistent assessment of atmospheric CO2 changes, ocean acidification and carbonate saturation state during this period. Here, we present a reconstruction of the Palaeocene–Eocene Thermal Maximum carbon cycle perturbation by assimilating seafloor sediment CaCO3 and sea surface temperature proxy data with simulations from an Earth system model, which includes a comprehensive carbonate system. Our reconstructions indicate a substantial increase in atmospheric CO2 from 890 ppm (95% credible interval: 680–1,170 ppm) to 1,980 ppm (1,680–2,280 ppm), coupled with a notable decline in pH (0.46 units, ranging from 0.31 to 0.63 units) and surface-water calcite saturation state, decreasing from 10.2 (7.5–12.8) in the pre-event period to 3.8 (2.8–5.1) during the thermal maximum. Carbonate undersaturation intensified substantially in high-latitude surface waters during the Palaeocene–Eocene Thermal Maximum, paralleling the current decline in Arctic aragonite saturation driven by anthropogenic CO2 emissions.

距今5600万年前的古新世-始新世热极盛期气候特征是碳的快速释放和海洋的广泛酸化。然而,我们对酸化和海洋饱和状态演变的理解仍然受到相当大的不确定性的阻碍,这主要源于代用数据的有限性。在这种情况下,数据同化可以对这一时期的大气二氧化碳变化、海洋酸化和碳酸盐饱和状态进行内部一致的评估。在这里,我们通过同化海底沉积物 CaCO3 和海面温度代用数据以及地球系统模型模拟结果,重建了古新世-始新世热极值碳循环扰动。我们的重建结果表明,大气中的二氧化碳含量从 890 ppm(95% 可信区间:680-1170 ppm)大幅增加到 1,980 ppm(1,680-2,280 ppm),同时 pH 值(0.46 个单位,从 0.31 个单位到 0.63 个单位不等)和表层水方解石饱和状态明显下降,从事件前时期的 10.2(7.5-12.8)下降到热极盛时期的 3.8(2.8-5.1)。在古新世-始新世热极值期间,高纬度表层水碳酸盐饱和度不足的情况大大加剧,与目前人为二氧化碳排放导致北极文石饱和度下降的情况类似。
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引用次数: 0
Estimated human-induced warming from a linear temperature and atmospheric CO2 relationship 根据温度与大气二氧化碳的线性关系估计人类引起的变暖
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-11 DOI: 10.1038/s41561-024-01580-5
Andrew Jarvis, Piers M. Forster

Assessing compliance with the human-induced warming goal in the Paris Agreement requires transparent, robust and timely metrics. Linearity between increases in atmospheric CO2 and temperature offers a framework that appears to satisfy these criteria, producing human-induced warming estimates that are at least 30% more certain than alternative methods. Here, for 2023, we estimate humans have caused a global increase of 1.49 ± 0.11 °C relative to a pre-1700 baseline.

评估《巴黎协定》中人类引起的气候变暖目标的遵守情况需要透明、可靠和及时的衡量标准。大气中二氧化碳的增加与温度的增加之间的线性关系提供了一个似乎能满足这些标准的框架,与其他方法相比,它产生的人类引起的变暖估计值至少要确定 30%。在此,我们估计 2023 年人类导致全球气温相对于 1700 年前的基线上升了 1.49 ± 0.11 °C。
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引用次数: 0
Frequent rainfall-induced new particle formation within the canopy in the Amazon rainforest 亚马逊雨林树冠内频繁降雨导致的新颗粒形成
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-08 DOI: 10.1038/s41561-024-01585-0
Luiz A. T. Machado, Gabriela R. Unfer, Sebastian Brill, Stefanie Hildmann, Christopher Pöhlker, Yafang Cheng, Jonathan Williams, Harder Hartwig, Meinrat O. Andreae, Paulo Artaxo, Joachim Curtius, Marco A. Franco, Micael A. Cecchini, Achim Edtbauer, Thorsten Hoffmann, Bruna Holanda, Théodore Khadir, Radovan Krejci, Leslie A. Kremper, Yunfan Liu, Bruno B. Meller, Mira L. Pöhlker, Carlos A. Quesada, Akima Ringsdorf, Ilona Riipinen, Susan Trumbore, Stefan Wolff, Jos Lelieveld, Ulrich Pöschl

Atmospheric aerosol particles are essential for forming clouds and precipitation, thereby influencing Earth’s energy budget, water cycle and climate on regional and global scales. However, the origin of aerosol particles over the Amazon rainforest during the wet season is poorly understood. Earlier studies showed new particle formation in the outflow of deep convective clouds and suggested a downward flux of aerosol particles during precipitation events. Here we use comprehensive aerosol, trace gas and meteorological data from the Amazon Tall Tower Observatory to show that rainfall regularly induces bursts of nanoparticles in the nucleation size range. This can be attributed to rain-related scavenging of larger particles and a corresponding reduction of the condensation sink, along with an ozone injection into the forest canopy, which could increase the oxidation of biogenic volatile organic compounds, especially terpenes, and enhance new particle formation. During and after rainfall, the nucleation particle concentrations directly above the canopy are greater than those higher up. This gradient persists throughout the wet season for the nucleation size range, indicating continuous particle formation within the canopy, a net upward flux of newly formed particles and a paradigm shift in understanding aerosol–cloud–precipitation interactions in the Amazon. Particle bursts provide a plausible explanation for the formation of cloud condensation nuclei, leading to the local formation of green-ocean clouds and precipitation. Our findings suggest that an interplay of a rain-related reduction in the condensation sink, primary emissions of gases, mainly terpenes, and particles from the forest canopy, and convective cloud processing determines the population of cloud condensation nuclei in pristine rainforest air.

大气气溶胶粒子对形成云层和降水至关重要,从而在区域和全球范围内影响地球的能量预算、水循环和气候。然而,人们对亚马逊雨林上空雨季气溶胶粒子的来源知之甚少。早期的研究表明,在深对流云的外流中会形成新的颗粒,并认为在降水事件中气溶胶颗粒会向下流动。在这里,我们利用亚马逊高塔观测站提供的综合气溶胶、痕量气体和气象数据表明,降雨会定期诱发成核粒径范围内的纳米粒子爆发。这可归因于与降雨有关的较大颗粒物的清除和冷凝汇的相应减少,以及向森林冠层注入臭氧,这可能会增加生物挥发性有机化合物(尤其是萜烯)的氧化,并促进新颗粒物的形成。在降雨期间和降雨之后,树冠正上方的成核粒子浓度要高于高处的成核粒子浓度。对于成核粒径范围而言,这种梯度在整个雨季都持续存在,表明冠层内颗粒物的形成是持续的,新形成的颗粒物是向上的净通量,亚马逊气溶胶-云-降水相互作用的理解范式发生了转变。粒子爆发为云凝结核的形成提供了一个合理的解释,从而导致当地形成绿色海洋云和降水。我们的研究结果表明,与降雨有关的凝结水汇减少、气体(主要是萜烯)和森林冠层颗粒物的一次排放以及对流云处理的相互作用,决定了原始雨林空气中云凝结核的数量。
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引用次数: 0
Carbon dioxide enrichment suppresses autotrophic nitrifiers in a rice ecosystem 富集二氧化碳可抑制水稻生态系统中的自养型硝化细菌
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-07 DOI: 10.1038/s41561-024-01590-3
Atmospheric CO2 enrichment inhibits the growth and activity of autotrophic nitrifiers through aggravation of anoxic stress in a nitrogen-rich paddy soil, according to a long-term free-air CO2 enrichment experiment. This CO2-induced inhibition effect on nitrifiers might contribute to the decline of inorganic nitrogen pools in lowland soil systems.
根据一项长期的自由空气二氧化碳富集实验,大气二氧化碳富集会通过加重富氮稻田土壤中的缺氧压力来抑制自养型硝化细菌的生长和活性。这种由二氧化碳引起的对硝化细菌的抑制作用可能会导致低地土壤系统中无机氮库的减少。
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引用次数: 0
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