New directions in sub-10-fs optical pulse generation

Sub-10-fs pulse generation has reached a maturity and robustness that gave rise to a rapid increase of new ultrafast applications. Some of these novel applications rely on the octave-spanning spectral width, the coherence properties, or the extremely high peak intensity of femtosecond lasers, which sets them apart from the traditional use of femtosecond lasers in ultrafast spectroscopy. In this review, we concentrate on the sub-10-fs regime and first discuss the state of the art in ultrashort pulse generation. We then report on ultrabroadband wavelength conversion schemes and dispersion control by chirped mirrors. We also review advances in pulse characterization methods, with which we can measure pulse properties with much higher accuracy than simple autocorrelation methods and which support even a bandwidth in the single-cycle regime. With the recent demonstrations of pulses with a duration of merely two optical cycles, a regime is entered where the relative phase between the carrier and the envelope of the pulse starts to play a role. We discuss methods to measure and control the carrier–envelope phase and point out applications in frequency metrology. A wealth of further novel directions and developments in femtosecond research is reviewed in this article.