{"title":"密闭蒸发介导的深层油藏悬浮水滴停留时间的延长","authors":"Naveen Puthussery Thrivikraman, Ashish Khare, Amit Sanjay Hegde, Anilakkad Raman Harikrishnan*","doi":"10.1021/acs.langmuir.1c02443","DOIUrl":null,"url":null,"abstract":"<p >We observe the impact of bouncing and floating of water drops on a pool of immiscible volatile oil pools at low Weber numbers. The residence time of the impacting drop ranges from a few milliseconds to a few seconds before it sinks into the lighter oil phase. It is hypothesized that the confined evaporation from the volatile oil pool replenishes the thin film draining and results in prolonged floating and delayed sinking of drops into the oil pool. Water drops are released from a low height to impact on volatile hydrocarbon oil deep pools of various volatilities. The floating dynamics and residence times are captured using high-speed imaging. A theoretical model for the residence time has been developed to evaluate the hypothesis. The drop residence time is found to be directly proportional to the volatility of the oil pool in accordance with the hypothesis. The mathematical model incorporating the coupled confined evaporation and film draining dynamics is found to be in well agreement with the experimentally observed residence time. The bouncing–sinking regime map has been developed based on the experimental data.</p>","PeriodicalId":50,"journal":{"name":"Langmuir","volume":null,"pages":null},"PeriodicalIF":3.7000,"publicationDate":"2021-11-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"6","resultStr":"{\"title\":\"Confined Evaporation-Mediated Enhanced Residence Time of Levitated Water Drops over Deep Oil Pools\",\"authors\":\"Naveen Puthussery Thrivikraman, Ashish Khare, Amit Sanjay Hegde, Anilakkad Raman Harikrishnan*\",\"doi\":\"10.1021/acs.langmuir.1c02443\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >We observe the impact of bouncing and floating of water drops on a pool of immiscible volatile oil pools at low Weber numbers. The residence time of the impacting drop ranges from a few milliseconds to a few seconds before it sinks into the lighter oil phase. It is hypothesized that the confined evaporation from the volatile oil pool replenishes the thin film draining and results in prolonged floating and delayed sinking of drops into the oil pool. Water drops are released from a low height to impact on volatile hydrocarbon oil deep pools of various volatilities. The floating dynamics and residence times are captured using high-speed imaging. A theoretical model for the residence time has been developed to evaluate the hypothesis. The drop residence time is found to be directly proportional to the volatility of the oil pool in accordance with the hypothesis. The mathematical model incorporating the coupled confined evaporation and film draining dynamics is found to be in well agreement with the experimentally observed residence time. The bouncing–sinking regime map has been developed based on the experimental data.</p>\",\"PeriodicalId\":50,\"journal\":{\"name\":\"Langmuir\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":3.7000,\"publicationDate\":\"2021-11-16\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"6\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Langmuir\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.langmuir.1c02443\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Langmuir","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.langmuir.1c02443","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Confined Evaporation-Mediated Enhanced Residence Time of Levitated Water Drops over Deep Oil Pools
We observe the impact of bouncing and floating of water drops on a pool of immiscible volatile oil pools at low Weber numbers. The residence time of the impacting drop ranges from a few milliseconds to a few seconds before it sinks into the lighter oil phase. It is hypothesized that the confined evaporation from the volatile oil pool replenishes the thin film draining and results in prolonged floating and delayed sinking of drops into the oil pool. Water drops are released from a low height to impact on volatile hydrocarbon oil deep pools of various volatilities. The floating dynamics and residence times are captured using high-speed imaging. A theoretical model for the residence time has been developed to evaluate the hypothesis. The drop residence time is found to be directly proportional to the volatility of the oil pool in accordance with the hypothesis. The mathematical model incorporating the coupled confined evaporation and film draining dynamics is found to be in well agreement with the experimentally observed residence time. The bouncing–sinking regime map has been developed based on the experimental data.
期刊介绍:
Langmuir is an interdisciplinary journal publishing articles in the following subject categories:
Colloids: surfactants and self-assembly, dispersions, emulsions, foams
Interfaces: adsorption, reactions, films, forces
Biological Interfaces: biocolloids, biomolecular and biomimetic materials
Materials: nano- and mesostructured materials, polymers, gels, liquid crystals
Electrochemistry: interfacial charge transfer, charge transport, electrocatalysis, electrokinetic phenomena, bioelectrochemistry
Devices and Applications: sensors, fluidics, patterning, catalysis, photonic crystals
However, when high-impact, original work is submitted that does not fit within the above categories, decisions to accept or decline such papers will be based on one criteria: What Would Irving Do?
Langmuir ranks #2 in citations out of 136 journals in the category of Physical Chemistry with 113,157 total citations. The journal received an Impact Factor of 4.384*.
This journal is also indexed in the categories of Materials Science (ranked #1) and Multidisciplinary Chemistry (ranked #5).