大气双射频介质阻挡放电非线性耦合的数值研究

Z. Zhang, Q. Nie, Z. Y. Wang, B. Jiang
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摘要

介质阻挡放电(DBD)作为一种在常压下产生高密度、低气体温度和丰富活性粒子等离子体的常用方法,在过去的几十年里得到了广泛的研究。其中,对等离子体参数调制的研究是一个新兴的研究热点。根据我们之前的双频驱动DBD的工作,已经证明了基于非线性频率耦合效应独立控制平均电子密度和气体温度的可能方法。本文采用一维流体模型和半动力学方法,系统地研究了双射频驱动DBD的非线性行为。根据有效电子能量分布函数(EEDF)和电子冲击电离率的结果,发现功率密度和相位关系的变化对电子密度、平均电子能和气体温度提供了单独的控制。此外,本文还讨论了模式转换。结果表明,等离子体鞘层中存在三种由非线性动力学控制的放电模式。其中,α模式的电离是由非线性耦合电子加热和局部瞬时电荷密度决定的。而在γ模式下,电离主要是由电子雪崩引起的。综上所述,双射频应用于DBD系统中,在两个频率之间产生非线性协同效应,为加强对等离子体参数的控制提供了一种可能的方法。
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Numerical Studies on the Nonlinear Coupling in Atmospheric Dual Radio-Frequency Dielectric Barrier Discharge
Dielectric barrier discharges (DBD) as a common method to generate plasmas with high density, low gas temperature, and abundant active particle under atmospheric pressure have been widely investigated in the past decades. Among these researches, the investigation on plasma parameters modulation represents a novel and budding focus. According to our previous works of DBD driven by dual-frequency, it has been demonstrated to provide a possible approach of controlling both averaged electron density and gas temperature independently based on the nonlinear frequency coupling effect. In this work, we used one-dimensional fluid model with semi-kinetic method, systemically studied the nonlinear behavior of the dual radio-frequency driven DBD. In term of the results of effective electron energy distribution function (EEDF) and electron impact ionization rate, it is found that the variations of power density and phase relationship provide separate control over the electron density, mean electron energy and gas temperature. Moreover, mode transitions are discussed in this paper. It is shown that there exist three kinds of discharge modes, which are governed by the nonlinear dynamics in the plasma sheath. Among which, the ionization in α mode is determined by the nonlinear coupling electron heating and local momentary charge density. While in γ mode, the ionization is caused mainly by the electron avalanches. In summary, the dual radio-frequency applied in DBD system is found to generate a nonlinear synergistic effect between two frequencies, which can provide a possible approach to enhance control over the plasma parameters.
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