Rajesh Sharma, K. Arnoult, Sunil Kumar Ramasahayam, Saad Azam, Zachary Hicks, A. Shaikh, T. Viswanathan
{"title":"新型碳基材料的光电化学制氢","authors":"Rajesh Sharma, K. Arnoult, Sunil Kumar Ramasahayam, Saad Azam, Zachary Hicks, A. Shaikh, T. Viswanathan","doi":"10.1109/IAS.2014.6978345","DOIUrl":null,"url":null,"abstract":"A transition to hydrogen as a major fuel could transform the US as well as global energy system increasing energy security while reducing environmental impact. This major transformation of our energy system would require a sustainable production of hydrogen using renewable resources. Hydrogen production using photo-electrochemical water splitting has been considered as a “holy grail” of sustainable hydrogen economy. Despite four decades of research since it was first shown that n-type TiO2 can be used for water splitting using sunlight, the search for a material that can efficiently harness solar energy for photo-electrolysis is still on. This paper will address some of the key challenges in the development of a material that is photoactive, stable, corrosion resistant and cost effective. This paper presents for the first time photo-electrochemical characterization of novel phosphorus, nitrogen doped carbon material (PNDC). The photocurrent density obtained was 0.416 mA/cm2, which is quite significant under visible radiation. This discovery opens up a large number of possibilities in development of a new class of carbon based materials for photo-electrochemical hydrogen production.","PeriodicalId":446068,"journal":{"name":"2014 IEEE Industry Application Society Annual Meeting","volume":"37 1","pages":"0"},"PeriodicalIF":0.0000,"publicationDate":"2014-12-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"2","resultStr":"{\"title\":\"Photo-electrochemical hydrogen production using novel carbon based material\",\"authors\":\"Rajesh Sharma, K. Arnoult, Sunil Kumar Ramasahayam, Saad Azam, Zachary Hicks, A. Shaikh, T. Viswanathan\",\"doi\":\"10.1109/IAS.2014.6978345\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"A transition to hydrogen as a major fuel could transform the US as well as global energy system increasing energy security while reducing environmental impact. This major transformation of our energy system would require a sustainable production of hydrogen using renewable resources. Hydrogen production using photo-electrochemical water splitting has been considered as a “holy grail” of sustainable hydrogen economy. Despite four decades of research since it was first shown that n-type TiO2 can be used for water splitting using sunlight, the search for a material that can efficiently harness solar energy for photo-electrolysis is still on. This paper will address some of the key challenges in the development of a material that is photoactive, stable, corrosion resistant and cost effective. This paper presents for the first time photo-electrochemical characterization of novel phosphorus, nitrogen doped carbon material (PNDC). The photocurrent density obtained was 0.416 mA/cm2, which is quite significant under visible radiation. This discovery opens up a large number of possibilities in development of a new class of carbon based materials for photo-electrochemical hydrogen production.\",\"PeriodicalId\":446068,\"journal\":{\"name\":\"2014 IEEE Industry Application Society Annual Meeting\",\"volume\":\"37 1\",\"pages\":\"0\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2014-12-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"2\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"2014 IEEE Industry Application Society Annual Meeting\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1109/IAS.2014.6978345\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"2014 IEEE Industry Application Society Annual Meeting","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1109/IAS.2014.6978345","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Photo-electrochemical hydrogen production using novel carbon based material
A transition to hydrogen as a major fuel could transform the US as well as global energy system increasing energy security while reducing environmental impact. This major transformation of our energy system would require a sustainable production of hydrogen using renewable resources. Hydrogen production using photo-electrochemical water splitting has been considered as a “holy grail” of sustainable hydrogen economy. Despite four decades of research since it was first shown that n-type TiO2 can be used for water splitting using sunlight, the search for a material that can efficiently harness solar energy for photo-electrolysis is still on. This paper will address some of the key challenges in the development of a material that is photoactive, stable, corrosion resistant and cost effective. This paper presents for the first time photo-electrochemical characterization of novel phosphorus, nitrogen doped carbon material (PNDC). The photocurrent density obtained was 0.416 mA/cm2, which is quite significant under visible radiation. This discovery opens up a large number of possibilities in development of a new class of carbon based materials for photo-electrochemical hydrogen production.