BaSO4:Eu纳米粒子作为高剂量不同电离辐射的探测器

N. Salah, S. Habib, Z. Khan, S. Lochab
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引用次数: 8

摘要

用48 MeV的7Li3+、75 MeV的C6+和90 MeV的O7+离子束在1 ~ 109 ~ 1 ~ 1013个离子/cm2的影响范围内照射了粒径约为40 nm的BaSO4:Eu荧光粉纳米粒子。记录并研究了辐照样品的热释光曲线。该样品的微晶形式包括在研究中,目的是报告比较测量。该材料在其纳米和微观形式暴露于60Co的伽马射线的TL结果也包括和更详细地研究。结果表明,纳米材料在离子作用下的发光曲线与伽玛射线作用下的发光曲线相似,在462 K处有一个剂量峰,旁边有一个较小的剂量峰,而在离子束和伽玛射线作用下的微晶样品在503 K处有一个明显的剂量峰,旁边有一个较小的剂量峰。观察到纳米晶材料在低通量/剂量下的TL灵敏度低于微晶样品,而在高通量/剂量下则高于微晶样品。这种纳米荧光粉在很宽的暴露范围内对高能离子和伽马辐射表现出线性/亚线性的TL响应,与微晶荧光粉相比,这种响应要宽得多。这使得BaSO4:Eu的纳米结构形式有助于估计用于放射治疗或食物/种子辐照的不同电离辐射的高剂量。
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The nanoparticles of BaSO4:Eu as detectors for high doses of different ionising radiations
Nanoparticles of a BaSO4:Eu phosphor with a particle size of around 40 nm have been irradiated by 48 MeV 7Li3+, 75 MeV C6+ and 90 MeV O7+ ion beams at the fluence range of 1 ∼ l09–1 ∼ 1013 ions/cm2. The thermoluminescence (TL) glow curves of the irradiated samples were recorded and studied. The microcrystalline form of this sample is included in the study with the aim of reporting a comparative measurement. The TL results of this material in its nano- and microforms exposed to the gamma rays of 60Co are also included and investigated in more detail. It is observed that the glow curves of the nanomaterial exposed to these ions are similar to that exposed to gamma rays, with a dosimetric peak at 462 K beside a smaller one at 503 K, while those of the microcrystalline sample exposed to both ion beams and gamma rays have their prominent peak at 503 K beside a smaller one at 462 K. The observed TL sensitivity of the nanocrystalline material is less than that of the microcrystalline sample at low fluences/doses, while it is more at higher fluences/doses. This nanophosphor exhibits a linear/sublinear TL response to energetic ions and gamma radiation over a very wide range of exposures, which is much wider compared to that of its microcrystalline counterpart. This makes the nanostructural form of BaSO4:Eu useful to estimate the high doses of different ionising radiations that are in use for radiotherapy or food/seed irradiation.
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