合理设计高效稳定的钙钛矿太阳能电池空穴传输层体系

IF 10.7 Q1 CHEMISTRY, PHYSICAL EcoMat Pub Date : 2023-09-26 DOI:10.1002/eom2.12414
Jaehee Lee, Taewoong Son, Kyeongbin Min, Seongjun Park, Youngwoong Kim, Jangwon Seo
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引用次数: 0

摘要

本文综述了钙钛矿太阳能电池(PSCs)空穴传输层(HTL)中有机/聚合物半导体的p型掺杂技术。首先,我们从掺杂剂和添加剂的角度研究了用于html的传统掺杂体系,以及它们的掺杂原理和局限性。其次,我们概述了目前克服传统掺杂剂体系局限性的研究策略:(i)大阳离子掺杂剂/添加剂,(ii)疏水性掺杂剂/添加剂,(iii)具有锁定能力的掺杂剂/添加剂,(iv)漂洗或离子交换方法,以及(v)其他方法。然后,我们提供了基于离子液体,路易斯酸,强受体等替代掺杂剂的综合分析。此外,综述了基于不同空穴输运材料、表面/界面处理和HTL结构修饰等多种研究方法的研究现状,并对高效稳定的psc所需HTL体系的发展进行了展望。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Rationally designed hole transporting layer system for efficient and stable perovskite solar cells

In this review, p-type doping technologies for organic/polymeric semiconductors in hole transporting layer (HTL) for perovskite solar cells (PSCs) are examined. Initially, we investigate the conventional dopant systems used for HTL in terms of dopants and additives, as well as their doping principles and limitations. Second, we recapitulate the current research strategies for overcoming the limitations of conventional dopant systems: (i) dopants/additives with large cations, (ii) hydrophobic dopants/additives, (iii) locking-capable dopants/additives, (iv) rinsing or ion exchange methods, and (v) other methods. Afterwards, we provide a comprehensive analysis of alternative dopants based on ionic liquids, Lewis acids, strong acceptors, and others. In addition, the review emphasizes current achievements based on multiple research approaches to diverse hole transporting materials, surface/interfacial treatment, and architectural modification of HTL, and provides a perspective on developments of desirable HTL system for efficient and stable PSCs.

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来源期刊
CiteScore
17.30
自引率
0.00%
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0
审稿时长
4 weeks
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