生物质衍生的碳纳米结构及其作为析氢和氧还原/析氢电催化剂的应用

Kristina Mikhailovna Maliutina, Joy Esohe Omoriyekomwan, Chuanxin He, Liangdong Fan, Andrea Folli
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引用次数: 0

摘要

合理设计活性、选择性和稳定性的生物质衍生电催化剂为燃料和增值化学品的电化学生产提供了一种主要的可持续途径。本文综述了生物质电催化纳米结构在氢析出反应(HER)和氧还原析出反应(氧还原反应和氧析出反应)领域的最新进展,这是主要研究工作的主题,也是公共和私人投资的主题,因为它们将在能源转型和实现净零碳排放中发挥关键作用。本文综述了可持续碳基纳米结构材料电催化性能的实验和理论研究,并为未来创新能源材料的商业化和应用提供了机会。在回顾相关文献的基础上,重点探讨了电催化活性/选择性与合成方法、组成、物理化学特性之间的关系,试图揭示其清晰的构效关系。此外,本研究针对不同电催化剂的催化机制、限制现象和可持续未来技术的实际应用进行了关键的比较。
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Biomass-derived carbon nanostructures and their applications as electrocatalysts for hydrogen evolution and oxygen reduction/evolution
Biomass derived electrocatalysts with rationally designed activity, selectivity, and stability present a major sustainable approach for the electrochemical production of fuels and value-added chemicals. This review presents recent advances in the field of biomass-derived electrocatalytic nanostructures for the hydrogen evolution reaction (HER) and the oxygen reduction and evolution reactions (oxygen reduction reaction and oxygen evolution reaction), that are subject of major research efforts, as well as public and private investment, as they will play a crucial role in the energy transition and in achieving net zero carbon emissions. The review summarises experimental and theoretical investigations aiming at tuning electrocatalytic performances of sustainable C-based nanostructured materials, and present opportunities for future commercialization of innovative energy materials and applications. In reviewing relevant literature in the field, we focus on the correlation between electrocatalytic activity/selectivity and synthesis methods, composition, physical chemical characteristics, in the attempt to uncover a clear structure-activity relationship. Furthermore, this study provides a critical comparison of the different electrocatalysts in light of their catalytic mechanisms, limiting phenomena, and practical applications for sustainable future technologies.
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