由于储层冲刷导致的甲烷排放:一个重要的排放途径?

IF 3.9 2区 地球科学 Q1 ECOLOGY Biogeosciences Pub Date : 2023-10-04 DOI:10.5194/bg-20-4057-2023
Ole Lessmann, Jorge Encinas Fernández, Karla Martínez-Cruz, Frank Peeters
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引用次数: 1

摘要

摘要水库是全球重要的温室气体甲烷(CH4)来源,它通过不同的排放途径排放。在一些水库中,水库冲刷被用作沉积物管理策略,以抵消威胁水库容量的日益增加的沉积物。水库冲淤利用了水位下降时水流的侵蚀力,通过大坝出水口将沉积物动员并输送到下游河流中。在这一过程中,沉积物中储存的CH4被释放到水中,并脱气到大气中,导致CH4排放。在这里,我们评估了这一CH4排放途径的重要性,并将其与储层中其他CH4排放途径进行了比较。我们测量了施瓦岑巴赫水库沉积物中CH4的季节和空间浓度,提供了淡水系统中最大的CH4孔隙水浓度数据集之一。基于该数据集,我们确定了沉积物的CH4通量,并估计了由于水库冲刷而产生的潜在CH4排放。由于一次冲洗操作而排放的甲烷占施瓦岑巴赫水库典型的年甲烷排放量的7% - 14%,因此释放的甲烷量取决于冲洗操作的季节时间,可能相差2倍。较大的冲刷事件调动了较深的沉积物层,导致CH4调动的非线性增加。这表明,较小沉积物层的定期冲刷释放的CH4少于较厚沉积物层较少冲刷事件中相同沉积物体积的去除量。然而,额外的间接甲烷排放途径对甲烷排放总量的贡献可能随着冲洗操作而变化。在其他沉积物负荷高于施瓦岑巴赫水库的水库中,水库冲洗可能会产生大量的甲烷排放,特别是在经常进行冲洗作业的情况下。我们的研究认识到由于水库冲刷造成的CH4排放是一个重要的途径,确定了减少这些CH4排放的潜在管理策略,并强调了进一步研究的必要性。
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Methane emissions due to reservoir flushing: a significant emission pathway?
Abstract. Reservoirs represent a globally significant source of the greenhouse gas methane (CH4), which is emitted via different emission pathways. In some reservoirs, reservoir flushing is employed as a sediment management strategy to counteract growing sediment deposits that threaten reservoir capacity. Reservoir flushing utilizes the eroding force of water currents during water level drawdown to mobilize and transport sediment deposits through the dam outlet into the downstream river. During this process, CH4 that is stored in the sediment can be released into the water and degas to the atmosphere, resulting in CH4 emissions. Here, we assess the significance of this CH4 emission pathway and compare it to other CH4 emission pathways from reservoirs. We measured seasonal and spatial CH4 concentrations in the sediment of Schwarzenbach Reservoir, providing one of the largest datasets on CH4 pore water concentrations in freshwater systems. Based on this dataset we determined CH4 fluxes from the sediment and estimated potential CH4 emissions due to reservoir flushing. CH4 emissions due to one flushing operation can constitute 7 %–14 % of the typical annual CH4 emissions from Schwarzenbach Reservoir, whereby the amount of released CH4 depends on the seasonal timing of the flushing operation and can differ by a factor of 2. Larger flushing events that mobilize deeper sediment layers lead to non-linear increases in CH4 mobilization. This suggests that regular flushing of smaller sediment layers releases less CH4 than removal of the same sediment volume in fewer flushing events of thicker sediment layers. However, additional indirect CH4 emissions pathways contributing to the total CH4 emissions may vary with the flushing operation. In other reservoirs with higher sediment loadings than Schwarzenbach Reservoir, reservoir flushing could cause substantial CH4 emissions, especially when flushing operations are conducted frequently. Our study recognizes CH4 emissions due to reservoir flushing as an important pathway, identifies potential management strategies to mitigate these CH4 emissions and emphasizes the need for further research.
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来源期刊
Biogeosciences
Biogeosciences 环境科学-地球科学综合
CiteScore
8.60
自引率
8.20%
发文量
258
审稿时长
4.2 months
期刊介绍: Biogeosciences (BG) is an international scientific journal dedicated to the publication and discussion of research articles, short communications and review papers on all aspects of the interactions between the biological, chemical and physical processes in terrestrial or extraterrestrial life with the geosphere, hydrosphere and atmosphere. The objective of the journal is to cut across the boundaries of established sciences and achieve an interdisciplinary view of these interactions. Experimental, conceptual and modelling approaches are welcome.
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