用于电催化制氢的铜、钯和还原石墨烯氧化物共掺杂层状 WS2/WO3 纳米结构

IF 2.1 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Electronic Materials Letters Pub Date : 2023-09-12 DOI:10.1007/s13391-023-00458-9
Vipin Kumar, Rajneesh Kumar Mishra, Le Gia Trung, Pushpendra Kumar, Sagar M. Mane, Jae Cheol Shin, Jin Seog Gwag
{"title":"用于电催化制氢的铜、钯和还原石墨烯氧化物共掺杂层状 WS2/WO3 纳米结构","authors":"Vipin Kumar,&nbsp;Rajneesh Kumar Mishra,&nbsp;Le Gia Trung,&nbsp;Pushpendra Kumar,&nbsp;Sagar M. Mane,&nbsp;Jae Cheol Shin,&nbsp;Jin Seog Gwag","doi":"10.1007/s13391-023-00458-9","DOIUrl":null,"url":null,"abstract":"<div><p>Fossil fuels have a vital role in global energy resources. The burning of fossil fuels produces pollutants and harms the environment. These environmental problems can be solved by searching for a substitute for fossil fuels. Hydrogen production by water electrolysis has emerged as a promising substitute. It is a green, clean, and renewable energy source. Low-cost water is abundant on the Earth. The metal and its composite material have been used to develop water electrolysis. Among these composite catalytic materials, WS<sub>2</sub>/WO<sub>3</sub> composite catalyst is well-known for its excellent physical and chemical behavior in water electrolysis to produce hydrogen. Engineered catalysts can further enhance the catalytic performance. Therefore, we investigate and analyze the catalytic performance of copper (Cu), palladium (Pd), and r-GO co-doped WS<sub>2</sub>/WO<sub>3</sub> composite material for water electrolysis to produce green, clean, and renewable hydrogen energy by hydrogen evolution reaction (HER). The hydrothermal synthesis method is used to prepare the WS<sub>2</sub>/WO<sub>3</sub> composite material co-doped with Cu, Pd, and r-GO. The co-doping is favorable for fast charge transfer by providing many active catalytic sites for HER and enhancing the HER catalytic performance. Therefore, the co-doped tungsten disulfide/oxide could be a potential composite material for efficient water electrolysis for clean and renewable hydrogen production by electrochemical water electrolysis.</p><h3>Graphical Abstract</h3>\n<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":536,"journal":{"name":"Electronic Materials Letters","volume":"20 4","pages":"414 - 424"},"PeriodicalIF":2.1000,"publicationDate":"2023-09-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Copper, Palladium, and Reduced Graphene Oxide Co-doped Layered WS2/WO3 Nanostructures for Electrocatalytic Hydrogen Generation\",\"authors\":\"Vipin Kumar,&nbsp;Rajneesh Kumar Mishra,&nbsp;Le Gia Trung,&nbsp;Pushpendra Kumar,&nbsp;Sagar M. Mane,&nbsp;Jae Cheol Shin,&nbsp;Jin Seog Gwag\",\"doi\":\"10.1007/s13391-023-00458-9\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Fossil fuels have a vital role in global energy resources. The burning of fossil fuels produces pollutants and harms the environment. These environmental problems can be solved by searching for a substitute for fossil fuels. Hydrogen production by water electrolysis has emerged as a promising substitute. It is a green, clean, and renewable energy source. Low-cost water is abundant on the Earth. The metal and its composite material have been used to develop water electrolysis. Among these composite catalytic materials, WS<sub>2</sub>/WO<sub>3</sub> composite catalyst is well-known for its excellent physical and chemical behavior in water electrolysis to produce hydrogen. Engineered catalysts can further enhance the catalytic performance. Therefore, we investigate and analyze the catalytic performance of copper (Cu), palladium (Pd), and r-GO co-doped WS<sub>2</sub>/WO<sub>3</sub> composite material for water electrolysis to produce green, clean, and renewable hydrogen energy by hydrogen evolution reaction (HER). The hydrothermal synthesis method is used to prepare the WS<sub>2</sub>/WO<sub>3</sub> composite material co-doped with Cu, Pd, and r-GO. The co-doping is favorable for fast charge transfer by providing many active catalytic sites for HER and enhancing the HER catalytic performance. Therefore, the co-doped tungsten disulfide/oxide could be a potential composite material for efficient water electrolysis for clean and renewable hydrogen production by electrochemical water electrolysis.</p><h3>Graphical Abstract</h3>\\n<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>\",\"PeriodicalId\":536,\"journal\":{\"name\":\"Electronic Materials Letters\",\"volume\":\"20 4\",\"pages\":\"414 - 424\"},\"PeriodicalIF\":2.1000,\"publicationDate\":\"2023-09-12\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Electronic Materials Letters\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s13391-023-00458-9\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Electronic Materials Letters","FirstCategoryId":"88","ListUrlMain":"https://link.springer.com/article/10.1007/s13391-023-00458-9","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

化石燃料在全球能源资源中发挥着至关重要的作用。化石燃料的燃烧会产生污染物,对环境造成危害。这些环境问题可以通过寻找化石燃料的替代品来解决。水电解制氢已成为一种前景广阔的替代品。它是一种绿色、清洁和可再生能源。地球上有大量低成本的水。金属及其复合材料已被用于开发水电解。在这些复合催化材料中,WS2/WO3 复合催化剂因其在电解水制氢过程中优异的物理和化学性能而闻名。工程催化剂可进一步提高催化性能。因此,我们研究并分析了铜(Cu)、钯(Pd)和r-GO共掺杂的WS2/WO3复合材料在水电解中的催化性能,以利用氢进化反应(HER)生产绿色、清洁和可再生的氢能。该研究采用水热合成法制备了共掺杂 Cu、Pd 和 r-GO 的 WS2/WO3 复合材料。共掺杂为 HER 提供了许多活性催化位点,有利于电荷的快速转移,从而提高 HER 的催化性能。因此,共掺杂的二硫化钨/氧化物可以成为一种潜在的复合材料,用于高效电解水,通过电化学电解水法生产清洁和可再生氢气。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

摘要图片

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Copper, Palladium, and Reduced Graphene Oxide Co-doped Layered WS2/WO3 Nanostructures for Electrocatalytic Hydrogen Generation

Fossil fuels have a vital role in global energy resources. The burning of fossil fuels produces pollutants and harms the environment. These environmental problems can be solved by searching for a substitute for fossil fuels. Hydrogen production by water electrolysis has emerged as a promising substitute. It is a green, clean, and renewable energy source. Low-cost water is abundant on the Earth. The metal and its composite material have been used to develop water electrolysis. Among these composite catalytic materials, WS2/WO3 composite catalyst is well-known for its excellent physical and chemical behavior in water electrolysis to produce hydrogen. Engineered catalysts can further enhance the catalytic performance. Therefore, we investigate and analyze the catalytic performance of copper (Cu), palladium (Pd), and r-GO co-doped WS2/WO3 composite material for water electrolysis to produce green, clean, and renewable hydrogen energy by hydrogen evolution reaction (HER). The hydrothermal synthesis method is used to prepare the WS2/WO3 composite material co-doped with Cu, Pd, and r-GO. The co-doping is favorable for fast charge transfer by providing many active catalytic sites for HER and enhancing the HER catalytic performance. Therefore, the co-doped tungsten disulfide/oxide could be a potential composite material for efficient water electrolysis for clean and renewable hydrogen production by electrochemical water electrolysis.

Graphical Abstract

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Electronic Materials Letters
Electronic Materials Letters 工程技术-材料科学:综合
CiteScore
4.70
自引率
20.80%
发文量
52
审稿时长
2.3 months
期刊介绍: Electronic Materials Letters is an official journal of the Korean Institute of Metals and Materials. It is a peer-reviewed international journal publishing print and online version. It covers all disciplines of research and technology in electronic materials. Emphasis is placed on science, engineering and applications of advanced materials, including electronic, magnetic, optical, organic, electrochemical, mechanical, and nanoscale materials. The aspects of synthesis and processing include thin films, nanostructures, self assembly, and bulk, all related to thermodynamics, kinetics and/or modeling.
期刊最新文献
Impact of Crystal Domain on Electrical Performance and Bending Durability of Flexible Organic Thin-Film Transistors with diF-TES-ADT Semiconductor All-Cobalt-Free Layered/Olivine Mixed Cathode Material for High-Electrode Density and Enhanced Cycle-Life Performance High-speed and Sub-ppm Detectable Tellurene NO2 Chemiresistive Room-Temperature Sensor under Humidity Environments A Neural Network Approach for Health State Estimation of Lithium-Ion Batteries Incorporating Physics Knowledge Enhanced Magnetic Permeability Through Improved Packing Density for Thin-Film Type Power Inductors for High-Frequency Applications
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1