将 CO2 电还原为 CO 的镍单原子催化剂的最新进展

Ziyan Yang, Rongzhen Chen, Ling Zhang, Yuhang Li and Chunzhong Li
{"title":"将 CO2 电还原为 CO 的镍单原子催化剂的最新进展","authors":"Ziyan Yang, Rongzhen Chen, Ling Zhang, Yuhang Li and Chunzhong Li","doi":"10.1039/D3IM00109A","DOIUrl":null,"url":null,"abstract":"<p>The electrocatalytic reduction of carbon dioxide (CO<small><sub>2</sub></small>) is considered an effective strategy for mitigating the energy crisis and the greenhouse effect. Nickel is widely used in single-atom catalysts (SACs) owing to its special electronic structure. In this minireview, the basic principles of Ni SACs in the electrocatalytic reduction of CO<small><sub>2</sub></small> to CO are first described. Subsequently, Ni SACs are divided into three categories depending on different strategies used to improve properties. The synthesis, morphology, performance and theoretical calculations of the catalysts are also described. Finally, an overview of the existing challenges and perspectives of Ni SACs for CO<small><sub>2</sub></small> reduction is presented.</p><p>Keywords: CO<small><sub>2</sub></small> reduction; Electrocatalysis; Nickel single-atom catalysts.</p>","PeriodicalId":29808,"journal":{"name":"Industrial Chemistry & Materials","volume":" 4","pages":" 533-555"},"PeriodicalIF":0.0000,"publicationDate":"2024-01-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.rsc.org/en/content/articlepdf/2024/im/d3im00109a?page=search","citationCount":"0","resultStr":"{\"title\":\"Recent progress in nickel single-atom catalysts for the electroreduction of CO2 to CO\",\"authors\":\"Ziyan Yang, Rongzhen Chen, Ling Zhang, Yuhang Li and Chunzhong Li\",\"doi\":\"10.1039/D3IM00109A\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The electrocatalytic reduction of carbon dioxide (CO<small><sub>2</sub></small>) is considered an effective strategy for mitigating the energy crisis and the greenhouse effect. Nickel is widely used in single-atom catalysts (SACs) owing to its special electronic structure. In this minireview, the basic principles of Ni SACs in the electrocatalytic reduction of CO<small><sub>2</sub></small> to CO are first described. Subsequently, Ni SACs are divided into three categories depending on different strategies used to improve properties. The synthesis, morphology, performance and theoretical calculations of the catalysts are also described. Finally, an overview of the existing challenges and perspectives of Ni SACs for CO<small><sub>2</sub></small> reduction is presented.</p><p>Keywords: CO<small><sub>2</sub></small> reduction; Electrocatalysis; Nickel single-atom catalysts.</p>\",\"PeriodicalId\":29808,\"journal\":{\"name\":\"Industrial Chemistry & Materials\",\"volume\":\" 4\",\"pages\":\" 533-555\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-01-09\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.rsc.org/en/content/articlepdf/2024/im/d3im00109a?page=search\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Industrial Chemistry & Materials\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2024/im/d3im00109a\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Industrial Chemistry & Materials","FirstCategoryId":"1085","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2024/im/d3im00109a","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0

摘要

电催化还原二氧化碳(CO2)被认为是缓解能源危机和温室效应的有效策略。镍因其特殊的电子结构而被广泛应用于单原子催化剂(SAC)中。在本小视图中,首先介绍了镍单原子催化剂在电催化将 CO2 还原成 CO 的过程中的基本原理。随后,根据改善性能的不同策略,Ni SACs 被分为三类。此外,还介绍了催化剂的合成、形态、性能和理论计算。最后,概述了用于二氧化碳还原的 Ni SACs 目前面临的挑战和前景。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

摘要图片

摘要图片

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Recent progress in nickel single-atom catalysts for the electroreduction of CO2 to CO

The electrocatalytic reduction of carbon dioxide (CO2) is considered an effective strategy for mitigating the energy crisis and the greenhouse effect. Nickel is widely used in single-atom catalysts (SACs) owing to its special electronic structure. In this minireview, the basic principles of Ni SACs in the electrocatalytic reduction of CO2 to CO are first described. Subsequently, Ni SACs are divided into three categories depending on different strategies used to improve properties. The synthesis, morphology, performance and theoretical calculations of the catalysts are also described. Finally, an overview of the existing challenges and perspectives of Ni SACs for CO2 reduction is presented.

Keywords: CO2 reduction; Electrocatalysis; Nickel single-atom catalysts.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Industrial Chemistry & Materials
Industrial Chemistry & Materials chemistry, chemical engineering, functional materials, energy, etc.-
自引率
0.00%
发文量
0
期刊介绍: Industrial Chemistry & Materials (ICM) publishes significant innovative research and major technological breakthroughs in all aspects of industrial chemistry and materials, with a particular focus on the important innovation of low-carbon chemical industry, energy and functional materials. By bringing researchers, engineers, and policymakers into one place, research is inspired, challenges are solved and the applications of science and technology are accelerated. The global editorial and advisory board members are valued experts in the community. With their support, the rigorous editorial practices and dissemination ensures your research is accessible and discoverable on a global scale. Industrial Chemistry & Materials publishes: ● Communications ● Full papers ● Minireviews ● Reviews ● Perspectives ● Comments
期刊最新文献
Back cover Membrane-free sequential paired electrosynthesis of 1,4-hydroquinone from phenol over a self-supported electrocatalytic electrode Back cover Toward a low-cost uranium-adsorbing material based on nonwoven fabrics and photografting technology Depolymerization of PET with Ethanol by Homogeneous Iron Catalysts Applied for Exclusive Chemical Recycling of Cloth Waste
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1