光催化二氧化碳还原新型材料的最新进展

Shanyue Lu, Shengwei Zhang, Qi Liu, Wen Wang, Ning Hao, Yajun Wang, Zhou Li, Dan Luo
{"title":"光催化二氧化碳还原新型材料的最新进展","authors":"Shanyue Lu,&nbsp;Shengwei Zhang,&nbsp;Qi Liu,&nbsp;Wen Wang,&nbsp;Ning Hao,&nbsp;Yajun Wang,&nbsp;Zhou Li,&nbsp;Dan Luo","doi":"10.1002/cnl2.107","DOIUrl":null,"url":null,"abstract":"<p>The conversion of CO<sub>2</sub> into chemical fuels, which can be stored and utilized through photocatalysis, represents an effective, environmentally friendly, and sustainable means to address both environmental concerns and energy shortages. CO<sub>2</sub>, as a stable oxidation product, poses challenges for reduction through light energy alone, necessitating the use of catalysts. Thus, a crucial aspect of CO<sub>2</sub> photocatalytic reduction technology lies in the development of effective photocatalysts. Based on the basic principle of PCRR (photocatalytic CO<sub>2</sub> reduction reaction), the review provides a detailed introduction to the core issues in PCRR process, including the relationship between band gap and catalyst reduction performance, effective utilization of photogenerated carriers, product selectivity, and methods for product analysis. Then, the recent research progresses of various photocatalysts are reviewed in the form of research examples combined with the above basic principles. Finally, this review summarizes and provides insights into the effective techniques for enhancing the photocatalytic activity of CO<sub>2</sub>, while also offering future prospects in this field.</p>","PeriodicalId":100214,"journal":{"name":"Carbon Neutralization","volume":"3 1","pages":"142-168"},"PeriodicalIF":0.0000,"publicationDate":"2024-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cnl2.107","citationCount":"0","resultStr":"{\"title\":\"Recent advances in novel materials for photocatalytic carbon dioxide reduction\",\"authors\":\"Shanyue Lu,&nbsp;Shengwei Zhang,&nbsp;Qi Liu,&nbsp;Wen Wang,&nbsp;Ning Hao,&nbsp;Yajun Wang,&nbsp;Zhou Li,&nbsp;Dan Luo\",\"doi\":\"10.1002/cnl2.107\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The conversion of CO<sub>2</sub> into chemical fuels, which can be stored and utilized through photocatalysis, represents an effective, environmentally friendly, and sustainable means to address both environmental concerns and energy shortages. CO<sub>2</sub>, as a stable oxidation product, poses challenges for reduction through light energy alone, necessitating the use of catalysts. Thus, a crucial aspect of CO<sub>2</sub> photocatalytic reduction technology lies in the development of effective photocatalysts. Based on the basic principle of PCRR (photocatalytic CO<sub>2</sub> reduction reaction), the review provides a detailed introduction to the core issues in PCRR process, including the relationship between band gap and catalyst reduction performance, effective utilization of photogenerated carriers, product selectivity, and methods for product analysis. Then, the recent research progresses of various photocatalysts are reviewed in the form of research examples combined with the above basic principles. Finally, this review summarizes and provides insights into the effective techniques for enhancing the photocatalytic activity of CO<sub>2</sub>, while also offering future prospects in this field.</p>\",\"PeriodicalId\":100214,\"journal\":{\"name\":\"Carbon Neutralization\",\"volume\":\"3 1\",\"pages\":\"142-168\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-01-22\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cnl2.107\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Carbon Neutralization\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/cnl2.107\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Carbon Neutralization","FirstCategoryId":"1085","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/cnl2.107","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0

摘要

通过光催化将二氧化碳转化为化学燃料并加以储存和利用,是解决环境问题和能源短缺的一种有效、环保和可持续的方法。二氧化碳作为一种稳定的氧化产物,仅靠光能进行还原是一项挑战,因此必须使用催化剂。因此,二氧化碳光催化还原技术的关键在于开发有效的光催化剂。本综述以 PCRR(光催化二氧化碳还原反应)的基本原理为基础,详细介绍了 PCRR 过程中的核心问题,包括带隙与催化剂还原性能的关系、光生载流子的有效利用、产物选择性以及产物分析方法。然后,结合上述基本原理,以研究实例的形式回顾了各种光催化剂的最新研究进展。最后,本综述对提高 CO2 光催化活性的有效技术进行了总结和深入分析,并对该领域的未来发展进行了展望。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

摘要图片

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Recent advances in novel materials for photocatalytic carbon dioxide reduction

The conversion of CO2 into chemical fuels, which can be stored and utilized through photocatalysis, represents an effective, environmentally friendly, and sustainable means to address both environmental concerns and energy shortages. CO2, as a stable oxidation product, poses challenges for reduction through light energy alone, necessitating the use of catalysts. Thus, a crucial aspect of CO2 photocatalytic reduction technology lies in the development of effective photocatalysts. Based on the basic principle of PCRR (photocatalytic CO2 reduction reaction), the review provides a detailed introduction to the core issues in PCRR process, including the relationship between band gap and catalyst reduction performance, effective utilization of photogenerated carriers, product selectivity, and methods for product analysis. Then, the recent research progresses of various photocatalysts are reviewed in the form of research examples combined with the above basic principles. Finally, this review summarizes and provides insights into the effective techniques for enhancing the photocatalytic activity of CO2, while also offering future prospects in this field.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
自引率
0.00%
发文量
0
期刊最新文献
Issue Information Front Cover: Carbon Neutralization, Volume 3, Issue 6, November 2024 Inside Back Cover Image: Carbon Neutralization, Volume 3, Issue 6, November 2024 Back Cover Image: Carbon Neutralization, Volume 3, Issue 6, November 2024 A chronicle of titanium niobium oxide materials for high-performance lithium-ion batteries: From laboratory to industry
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1