{"title":"通过高能电子散射研究氪的广义振子强度和积分截面","authors":"Wan-Lu Ma, Shu-Xing Wang, Zhi-Wei Nie, Jian-Hui Zhu, Jin-Feng Chen, Lin-Fan Zhu","doi":"10.1016/j.elspec.2024.147422","DOIUrl":null,"url":null,"abstract":"<div><p>Absolute generalized oscillator strengths of the valence-shell excitations of krypton have been determined with an incident electron energy of 1500 eV and an energy resolution of about 80 meV. By employing the relative flow technique with a dilute target, the pressure effect is excluded and the accuracy of the measured generalized oscillator strengths is improved. By comparing the present generalized oscillator strengths with the previous experimental and theoretical results, it is found that the first Born approximation is not reached at the squared momentum transfer larger than 1 a.u.. The optical oscillator strengths have been obtained by extrapolating the measured generalized oscillator strengths to zero squared momentum transfer, which cross-checks the previous electron impact and photoabsorption results. With the aid of the BE-scaling method, the integral cross sections of krypton have been determined from the excitation threshold to 5000 eV. The present oscillator strengths and integral cross sections supplement the fundamental database of the electron scattering of krypton and provide a benchmark for the theoretical methods.</p></div>","PeriodicalId":15726,"journal":{"name":"Journal of Electron Spectroscopy and Related Phenomena","volume":"271 ","pages":"Article 147422"},"PeriodicalIF":1.8000,"publicationDate":"2024-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Generalized oscillator strengths and integral cross sections of krypton studied by high-energy electron scattering\",\"authors\":\"Wan-Lu Ma, Shu-Xing Wang, Zhi-Wei Nie, Jian-Hui Zhu, Jin-Feng Chen, Lin-Fan Zhu\",\"doi\":\"10.1016/j.elspec.2024.147422\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Absolute generalized oscillator strengths of the valence-shell excitations of krypton have been determined with an incident electron energy of 1500 eV and an energy resolution of about 80 meV. By employing the relative flow technique with a dilute target, the pressure effect is excluded and the accuracy of the measured generalized oscillator strengths is improved. By comparing the present generalized oscillator strengths with the previous experimental and theoretical results, it is found that the first Born approximation is not reached at the squared momentum transfer larger than 1 a.u.. The optical oscillator strengths have been obtained by extrapolating the measured generalized oscillator strengths to zero squared momentum transfer, which cross-checks the previous electron impact and photoabsorption results. With the aid of the BE-scaling method, the integral cross sections of krypton have been determined from the excitation threshold to 5000 eV. The present oscillator strengths and integral cross sections supplement the fundamental database of the electron scattering of krypton and provide a benchmark for the theoretical methods.</p></div>\",\"PeriodicalId\":15726,\"journal\":{\"name\":\"Journal of Electron Spectroscopy and Related Phenomena\",\"volume\":\"271 \",\"pages\":\"Article 147422\"},\"PeriodicalIF\":1.8000,\"publicationDate\":\"2024-01-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Electron Spectroscopy and Related Phenomena\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0368204824000057\",\"RegionNum\":4,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"SPECTROSCOPY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Electron Spectroscopy and Related Phenomena","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0368204824000057","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"SPECTROSCOPY","Score":null,"Total":0}
引用次数: 0
摘要
在入射电子能量为 1500 eV、能量分辨率约为 80 meV 的条件下,测定了氪价壳激发的绝对广义振荡器强度。通过使用稀释目标的相对流技术,排除了压力效应,提高了测量广义振荡器强度的精度。通过将目前的广义振荡器强度与之前的实验和理论结果进行比较,发现在动量传递平方大于 1 a.u. 时并没有达到第一玻恩近似。光学振荡器强度是通过将测量到的广义振荡器强度外推到零平方动量传递得到的,这与之前的电子撞击和光吸收结果进行了交叉检验。借助 BE 缩放法,确定了从激发阈值到 5000 eV 的氪积分截面。目前的振子强度和积分截面补充了氪电子散射的基础数据库,并为理论方法提供了基准。
Generalized oscillator strengths and integral cross sections of krypton studied by high-energy electron scattering
Absolute generalized oscillator strengths of the valence-shell excitations of krypton have been determined with an incident electron energy of 1500 eV and an energy resolution of about 80 meV. By employing the relative flow technique with a dilute target, the pressure effect is excluded and the accuracy of the measured generalized oscillator strengths is improved. By comparing the present generalized oscillator strengths with the previous experimental and theoretical results, it is found that the first Born approximation is not reached at the squared momentum transfer larger than 1 a.u.. The optical oscillator strengths have been obtained by extrapolating the measured generalized oscillator strengths to zero squared momentum transfer, which cross-checks the previous electron impact and photoabsorption results. With the aid of the BE-scaling method, the integral cross sections of krypton have been determined from the excitation threshold to 5000 eV. The present oscillator strengths and integral cross sections supplement the fundamental database of the electron scattering of krypton and provide a benchmark for the theoretical methods.
期刊介绍:
The Journal of Electron Spectroscopy and Related Phenomena publishes experimental, theoretical and applied work in the field of electron spectroscopy and electronic structure, involving techniques which use high energy photons (>10 eV) or electrons as probes or detected particles in the investigation.