利用氧化锌负载碳纤维增强废水中土霉素抗生素的光降解。

IF 1.4 4区 农林科学 Q4 ENVIRONMENTAL SCIENCES Journal of Environmental Science and Health Part B-pesticides Food Contaminants and Agricultural Wastes Pub Date : 2024-01-01 Epub Date: 2024-02-21 DOI:10.1080/03601234.2024.2317678
Trung Hieu Bui, Dang Manh Le, Duc Anh Dinh, Huong Pham Thi
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引用次数: 0

摘要

抗生素土霉素(OCA)在自然环境中具有很高的不溶性,对其去除构成了巨大挑战。本研究合成了一种多孔结构和高表面积碳纤维,并将氧化锌(ZnO/CFB)融入其中,以有效去除废水中的土霉素。材料表征显示 ZnO/CFB 具有优异的光学和光化学特性,其带隙能降低至 2.7 eV。ZnO/CFB 在光降解废水中的 OCA 方面表现出强劲的性能,达到了令人印象深刻的 86.7% 的去除率。值得注意的是,总有机碳(TOC)的降低率达到了 97.5%。LC-MS 分析证实,OCA 及其中间产物在 60 分钟内被完全氧化,转化为无机物。这项研究介绍了一种消除废水中抗生素污染物的有效策略,凸显了 ZnO/CFB 作为一种有效、稳定的光催化剂在环境修复方面的潜力。
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Enhanced photodegradation of oxytetracycline antibiotic in wastewater by implementing ZnO-loaded carbon fiber.

The antibiotic oxytetracycline (OCA) exhibits high insolubility in the natural environment, posing a significant challenge for its removal. This study synthesized a porous structure and a high-surface-area carbon fiber, incorporating zinc oxide (ZnO/CFB) for the effective removal of OCA in wastewater. The material characterization revealed exceptional optical and photochemical properties of ZnO/CFB, featuring a reduced band gap energy of 2.7 eV. ZnO/CFB exhibited robust performance in the photodegradation of OCA in wastewater, achieving an impressive removal efficiency of 86.7%. Remarkably, the reduction of total organic carbon (TOC) reached an outstanding 97.5%. LC-MS analysis confirmed the complete oxidation of OCA and its intermediates, transforming them into inorganic substances within 60 min. This study introduces an efficient strategy for eliminating antibiotic pollutants from wastewater, highlighting the potential of ZnO/CFB as an effective and stable photocatalyst for environmental remediation.

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来源期刊
CiteScore
4.00
自引率
5.00%
发文量
87
审稿时长
1 months
期刊介绍: 12 issues per year Abstracted/indexed in: Agricola; Analytical Abstracts; ASFA 3: Aquatic Pollution & Environmental Quality; BioSciences Information Service of Biological Abstracts (BIOSIS); CAB Abstracts; CAB AGBiotech News and Information; CAB Irrigation & Drainage Abstracts; CAB Soils & Fertilizers Abstracts; Chemical Abstracts Service Plus; CSA Aluminum Industry Abstracts; CSA ANTE: Abstracts in New Technology and Engineering; CSA ASFA 3 Aquatic Pollution and Environmental Quality; CSA ASSIA: Applied Social Sciences Index & Abstracts; CSA Ecology Abstracts; CSA Entomology Abstracts; CSA Environmental Engineering Abstracts; CSA Health & Safety Science Abstracts; CSA Pollution Abstracts; CSA Toxicology Abstracts; CSA Water Resource Abstracts; EBSCOhost Online Research Databases; Elsevier BIOBASE/Current Awareness in Biological Sciences; Elsevier Engineering Information: EMBASE/Excerpta Medica/ Engineering Index/COMPENDEX PLUS; Environment Abstracts; Environmental Knowledge; Food Science and Technology Abstracts; Geo Abstracts; Geobase; Food Science; Index Medicus/ MEDLINE; INIST-Pascal/ CNRS; NIOSHTIC; ISI BIOSIS Previews; Pesticides; Food Contaminants and Agricultural Wastes: Analytical Abstracts; Pollution Abstracts; PubSCIENCE; Reference Update; Research Alert; Science Citation Index Expanded (SCIE); and Water Resources Abstracts.
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