根据 H2-SCR 催化剂的促进剂和支持类型同时减少 NOX 和 CO 有害气体

IF 1.5 4区 工程技术 Q3 ENGINEERING, MECHANICAL International Journal of Automotive Technology Pub Date : 2024-02-20 DOI:10.1007/s12239-024-00006-w
Choong-kil Seo
{"title":"根据 H2-SCR 催化剂的促进剂和支持类型同时减少 NOX 和 CO 有害气体","authors":"Choong-kil Seo","doi":"10.1007/s12239-024-00006-w","DOIUrl":null,"url":null,"abstract":"<p>The purpose of this study is to simultaneously reduce NO<sub>X</sub> and CO harmful gases according to the promoters and support types of the H<sub>2</sub>-SCR. The 0.5Pt-2CeO<sub>2</sub>-5Ru/TiO<sub>2</sub> catalyst loaded with 7 wt% Ru showed a lower NO<sub>X</sub> conversion rate compared to than the 0.5Pt-2CeO<sub>2</sub>/TiO<sub>2</sub> (STD), but the window shifted to the right, and it showed NO<sub>X</sub> reduction performance of up to 30% at 175 °C. When Zr was loaded, de- NO<sub>X</sub> performance was not improved at the temperature of 200 °C starting from a low catalyst temperature of 75 °C. With in the influence of the support types, the 0.5Pt-2CeO<sub>2</sub>/TiO<sub>2</sub> H<sub>2</sub>-SCR catalyst showed the highest NO<sub>X</sub> conversion rate below 125 °C, and the low-temperature activity of NO<sub>X</sub> was higher than that of the three zeolite-loaded H<sub>2</sub>-SCR catalysts. Low temperature activity was improved because the TiO<sub>2</sub> has excellent reducing and oxidizing ability. Among the three zeolites, the CO reduction performance of the 0.5Pt-2CeO<sub>2</sub>/Zeolite (1) catalyst with high Al content was the lowest.</p>","PeriodicalId":50338,"journal":{"name":"International Journal of Automotive Technology","volume":"188 1","pages":""},"PeriodicalIF":1.5000,"publicationDate":"2024-02-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Simultaneous Reduction of NOX and CO Harmful Gases According to the Promoters and Support Types of H2-SCR Catalyst\",\"authors\":\"Choong-kil Seo\",\"doi\":\"10.1007/s12239-024-00006-w\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The purpose of this study is to simultaneously reduce NO<sub>X</sub> and CO harmful gases according to the promoters and support types of the H<sub>2</sub>-SCR. The 0.5Pt-2CeO<sub>2</sub>-5Ru/TiO<sub>2</sub> catalyst loaded with 7 wt% Ru showed a lower NO<sub>X</sub> conversion rate compared to than the 0.5Pt-2CeO<sub>2</sub>/TiO<sub>2</sub> (STD), but the window shifted to the right, and it showed NO<sub>X</sub> reduction performance of up to 30% at 175 °C. When Zr was loaded, de- NO<sub>X</sub> performance was not improved at the temperature of 200 °C starting from a low catalyst temperature of 75 °C. With in the influence of the support types, the 0.5Pt-2CeO<sub>2</sub>/TiO<sub>2</sub> H<sub>2</sub>-SCR catalyst showed the highest NO<sub>X</sub> conversion rate below 125 °C, and the low-temperature activity of NO<sub>X</sub> was higher than that of the three zeolite-loaded H<sub>2</sub>-SCR catalysts. Low temperature activity was improved because the TiO<sub>2</sub> has excellent reducing and oxidizing ability. Among the three zeolites, the CO reduction performance of the 0.5Pt-2CeO<sub>2</sub>/Zeolite (1) catalyst with high Al content was the lowest.</p>\",\"PeriodicalId\":50338,\"journal\":{\"name\":\"International Journal of Automotive Technology\",\"volume\":\"188 1\",\"pages\":\"\"},\"PeriodicalIF\":1.5000,\"publicationDate\":\"2024-02-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"International Journal of Automotive Technology\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1007/s12239-024-00006-w\",\"RegionNum\":4,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENGINEERING, MECHANICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"International Journal of Automotive Technology","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1007/s12239-024-00006-w","RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENGINEERING, MECHANICAL","Score":null,"Total":0}
引用次数: 0

摘要

本研究的目的是根据 H2-SCR 的促进剂和载体类型,同时减少 NOX 和 CO 有害气体。与 0.5Pt-2CeO2/TiO2 催化剂(STD)相比,负载 7 wt% Ru 的 0.5Pt-2CeO2-5Ru/TiO2 催化剂的 NOX 转化率较低,但窗口向右移动,在 175 ℃ 时 NOX 减排性能高达 30%。当负载 Zr 时,从 75 ℃ 的低催化剂温度开始,在 200 ℃ 的温度下,脱 NOX 性能没有得到改善。受载体类型的影响,0.5Pt-2CeO2/TiO2 H2-SCR 催化剂在 125 ℃ 以下的 NOX 转化率最高,NOX 的低温活性也高于三种沸石负载型 H2-SCR 催化剂。低温活性提高的原因是 TiO2 具有优异的还原和氧化能力。在三种沸石中,高铝含量的 0.5Pt-2CeO2/ 沸石 (1) 催化剂的 CO 还原性能最低。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

摘要图片

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Simultaneous Reduction of NOX and CO Harmful Gases According to the Promoters and Support Types of H2-SCR Catalyst

The purpose of this study is to simultaneously reduce NOX and CO harmful gases according to the promoters and support types of the H2-SCR. The 0.5Pt-2CeO2-5Ru/TiO2 catalyst loaded with 7 wt% Ru showed a lower NOX conversion rate compared to than the 0.5Pt-2CeO2/TiO2 (STD), but the window shifted to the right, and it showed NOX reduction performance of up to 30% at 175 °C. When Zr was loaded, de- NOX performance was not improved at the temperature of 200 °C starting from a low catalyst temperature of 75 °C. With in the influence of the support types, the 0.5Pt-2CeO2/TiO2 H2-SCR catalyst showed the highest NOX conversion rate below 125 °C, and the low-temperature activity of NOX was higher than that of the three zeolite-loaded H2-SCR catalysts. Low temperature activity was improved because the TiO2 has excellent reducing and oxidizing ability. Among the three zeolites, the CO reduction performance of the 0.5Pt-2CeO2/Zeolite (1) catalyst with high Al content was the lowest.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
International Journal of Automotive Technology
International Journal of Automotive Technology 工程技术-工程:机械
CiteScore
3.10
自引率
12.50%
发文量
129
审稿时长
6 months
期刊介绍: The International Journal of Automotive Technology has as its objective the publication and dissemination of original research in all fields of AUTOMOTIVE TECHNOLOGY, SCIENCE and ENGINEERING. It fosters thus the exchange of ideas among researchers in different parts of the world and also among researchers who emphasize different aspects of the foundations and applications of the field. Standing as it does at the cross-roads of Physics, Chemistry, Mechanics, Engineering Design and Materials Sciences, AUTOMOTIVE TECHNOLOGY is experiencing considerable growth as a result of recent technological advances. The Journal, by providing an international medium of communication, is encouraging this growth and is encompassing all aspects of the field from thermal engineering, flow analysis, structural analysis, modal analysis, control, vehicular electronics, mechatronis, electro-mechanical engineering, optimum design methods, ITS, and recycling. Interest extends from the basic science to technology applications with analytical, experimental and numerical studies. The emphasis is placed on contributions that appear to be of permanent interest to research workers and engineers in the field. If furthering knowledge in the area of principal concern of the Journal, papers of primary interest to the innovative disciplines of AUTOMOTIVE TECHNOLOGY, SCIENCE and ENGINEERING may be published. Papers that are merely illustrations of established principles and procedures, even though possibly containing new numerical or experimental data, will generally not be published. When outstanding advances are made in existing areas or when new areas have been developed to a definitive stage, special review articles will be considered by the editors. No length limitations for contributions are set, but only concisely written papers are published. Brief articles are considered on the basis of technical merit.
期刊最新文献
Testbed and Analysis of Highway Cut-In Scenarios for Evaluating the AEB and FCW Functions Prediction Models of Overall Thermal Sensation and Comfort in Vehicle Cabin Based on Field Experiments Efficient Path Planning for Automated Valet Parking: Integrating Hybrid A* Search with Geometric Curves Road Feel Simulation Method with Rack Force Observer for Intelligent Vehicle Steer-by-Wire System Multi-physical Field Coupling Analysis of Flat Wire Motor
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1