{"title":"通过拉盖尔高斯束在分子磁体上诱导扭矩","authors":"Gang Lei, Shanzhi Li","doi":"10.1088/1612-202x/ad3623","DOIUrl":null,"url":null,"abstract":"This theoretical study delves into the induction of torque by light beams carrying orbital angular momentum on single-molecule magnets (SMMs). The investigation explores the impact of decay rates, detunings, and control field intensities on the generation of light-induced torque and the resulting current flow in a ring formation. The results highlight the crucial role of the control field, showcasing its efficacy as a tool to manipulate and amplify torque at different frequencies. Detuning is identified as a critical parameter influencing the shift, slope, and emergence of multiple peaks in the torque profile. The interplay between detuning, control field intensity, and decay rates introduces a control mechanism for fine-tuning torque at distinct probe frequencies. These findings underscore the potential applications of the control field and detuning as robust tools for tailored manipulation of torque in SMMs, paving the way for advancements in controlled current flow dynamics with ring structures.","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2024-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Inducing torque on molecular magnets via Laguerre Gaussian beams\",\"authors\":\"Gang Lei, Shanzhi Li\",\"doi\":\"10.1088/1612-202x/ad3623\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"This theoretical study delves into the induction of torque by light beams carrying orbital angular momentum on single-molecule magnets (SMMs). The investigation explores the impact of decay rates, detunings, and control field intensities on the generation of light-induced torque and the resulting current flow in a ring formation. The results highlight the crucial role of the control field, showcasing its efficacy as a tool to manipulate and amplify torque at different frequencies. Detuning is identified as a critical parameter influencing the shift, slope, and emergence of multiple peaks in the torque profile. The interplay between detuning, control field intensity, and decay rates introduces a control mechanism for fine-tuning torque at distinct probe frequencies. These findings underscore the potential applications of the control field and detuning as robust tools for tailored manipulation of torque in SMMs, paving the way for advancements in controlled current flow dynamics with ring structures.\",\"PeriodicalId\":1,\"journal\":{\"name\":\"Accounts of Chemical Research\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":16.4000,\"publicationDate\":\"2024-03-27\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Accounts of Chemical Research\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1088/1612-202x/ad3623\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1088/1612-202x/ad3623","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Inducing torque on molecular magnets via Laguerre Gaussian beams
This theoretical study delves into the induction of torque by light beams carrying orbital angular momentum on single-molecule magnets (SMMs). The investigation explores the impact of decay rates, detunings, and control field intensities on the generation of light-induced torque and the resulting current flow in a ring formation. The results highlight the crucial role of the control field, showcasing its efficacy as a tool to manipulate and amplify torque at different frequencies. Detuning is identified as a critical parameter influencing the shift, slope, and emergence of multiple peaks in the torque profile. The interplay between detuning, control field intensity, and decay rates introduces a control mechanism for fine-tuning torque at distinct probe frequencies. These findings underscore the potential applications of the control field and detuning as robust tools for tailored manipulation of torque in SMMs, paving the way for advancements in controlled current flow dynamics with ring structures.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.