强低频声波下的表面活性气泡动力学特性研究

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2024-04-27 DOI:10.1007/s12217-024-10101-3
Yun Zhao, Ruiqi Huang, Yong Chen, Qi Feng
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引用次数: 0

摘要

本文深入探讨了表面活性气泡在低频声波作用下的动力学特性,重点研究了气泡的稳定性效应和破裂的基本原理。根据实际生物数据对 Rayleigh-Plesset 方程进行了扩展和修改,从而建立了一个具有非线性表面张力的表面活性气泡模型。利用 Runge-Kutta 方法进行数值计算,发现声波振幅越大,气泡振幅越大。声波频率只在低频范围内影响气泡振动频率,但在共振频率下,气泡振荡剧烈。为了进一步解释气泡破裂,研究了气泡表面活性层的应力-应变关系,气泡壁上的应力随着气泡半径的增加而急剧增加。表面活性气泡非球形界面的稳定性揭示了一个临界半径值,当半径小于该值时,气泡处于稳定状态。通过模拟观察发现,气泡在稳定状态下振动,但当半径超过临界值时,会出现非球形界面,最终导致气泡向内凹陷和破裂。
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Study on Surface Active Bubble Dynamics Properties under Strong Low-Frequency Sound Waves

This paper delves into the dynamics of surface-active bubbles under low-frequency acoustic waves, with a focus on the stability effect and basic principle of rupture. The Rayleigh-Plesset equation is extended and modified based on real biological data, resulting in a model of surface-active bubbles with nonlinear surface tension. Using the Runge-Kutta method for numerical calculations, it is observed that larger acoustic wave amplitudes lead to larger bubble amplitudes. The acoustic wave frequency only affects the bubble vibration frequency in the low-frequency range, but at the resonance frequency, the bubble oscillations are violent. To further explain bubble rupture, the stress-strain relationship of the surface active layer of the bubble is studied, with the stress on the wall increasing sharply with the bubble radius. The stability of the non-spherical interface of the surface-active bubbles reveals a critical radius value, with bubbles in a stable state when the radius is smaller than this value. Through simulation, it is observed that bubbles vibrate in a steady state under stable conditions, but when the radius exceeds the critical value, a non-spherical interface appears ultimately resulting in inward depression and rupture.

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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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